持久性有机污染物在多介质中的分布及环境行为
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摘要
持久性有机污物(Persistent Organic Pollutants,POPs),具有长期残留性、半挥发性、生物蓄积性、高毒性,严重危害环境和人类健康,已成为全球性环境问题,受到全球高度关注。了解持久性有机污染物在多介质中的分布及环境行为,根据其来源、分布、转化行为、归宿规律可制定更好的POPs污染控制策略及有效治理途径,对POPs污染的控制、治理及去除具有重要意义。本文综述了POPs在水体、沉积物、土壤、大气中及生物体内的来源、分布、迁移、转化机理、富集及对人类健康的危害,并对POPs污染防治、治理及消除提出意见和对策。
引文
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[3]Zhang K,Zhang B Z,Li S M,et al.Regional dynamics of persistent organic pollutants(POPs)in the Pearl River Delta,China:Implications and perspectives[J].Environmental Pollution,2011,159(10):2301-2309.
[4]余刚,黄俊.持久性有机污染物知识100问[M].北京:中国环境科学出版社,2005.
[5]王亚鞯,蔡亚岐,江桂斌.斯德哥尔摩公约新增持久性有机污染物的一些研究进展[J].中国科学.化学,2010,40(2):99—123.
[6]余刚,牛军峰,黄俊,等.持久性有机污染物——新的全球性环境问题[M].北京:科学出版社,2005.
[7]Bao L J,Keith A M,Shane A S,et al.China's water pollution by persistent organic pollutants[J].Environmental Pollution,2012,163:100-108.
[8]马万里,刘丽艳,齐虹,等.松花江流域冰封期水体中多环芳烃的污染特征研究[J].环境科学,2012,33(12):4420-4425.
[9]Li G C,Xia X H,Wang R,et al.Pollution of polycyclic aromatic hydrocarbons(PAHs)in middle and lower reaches of the Yellow River[J].Environmental Science,2006,27(9):1738-1743.
[10]李秀丽,赖子尼,穆三妞,等.珠江入海口表层沉积物中多氯联苯残留与风险评价[J].生态环境学报,2012,21(12):135-140.
[11]冯承莲,夏星辉,周追,等.长江武汉段水体中多环芳烃的分布及来源分析[J].环境科学学报,2007,27(11):1900—1908.
[12]康跃惠,刘培斌,王子健,等.北京官厅水库—永定河水系水体中持久性有机氯农药污染[J].湖泊科学,2003,15(2):125—132.
[13]张伟玲,张干,祁士华,等.西藏错鄂湖和羊卓雍湖水体及沉积物中有机氯农药的初步研究[J].地球化学,2003,32(4):363—367.
[14]胡国成,郑海,张丽娟,等.珠江三角洲土壤中全氟化合物污染特征研究[J].中国环境科学,2013,33(S1):37-42.
[15]陈燕燕,尹颖,王晓蓉等.太湖表层沉积物中PAHs和PCBs的分布及风险评价[J].中国环境科学,2009,29(2):118—124.
[16]林田,马传良,王丽芳,等.滇池沉积物中多氯联苯和有机氯农药的残留特征与风险评估[J].地球与环境,2014,42(5):625—630.
[17]Guo Jian yang,Wu Feng chang,Liao Hai qing,et al.Sedimentary record of polycyclic aromatic hydrocarbons and DDTs in Dianchi Lake,an urban lake in Southwest China[J].Environmental Science and Pollution Research,2013,20(8):5471-5480.
[18]张帆,余应新,张东平,等.溴系阻燃剂在环境及人体中的存在和代谢转化[J].化学进展,2009,21(6):1364-1372.
[19]胡吉成.北京市大气中涣代阻燃刊环境行为的研究[M].中央民族大学,2010.
[20]Cooney C M.Detecting a new PCB in Chicago air[J].EnvironSciTechnol,2009,43(1):4-4.
[21]戴朝霞,陈振翔,王格慧,等.典型城市大气颗粒物中多环芳烃的污染研究[J].环境科学与技术,2006,2.
[22]Meijer S N,Ockenden W A,Sweetman A,et al.Global distribution and budget of PCBs and HCB in background surface soils:Implications for sources and environmental processes[J].Environmental Science&Technology,2003,37(4):667-672.
[23]崔嵩,杨萌,李一凡.不同土壤类型多氯联苯土壤残留特征变化分析[J].吉林大学学报(地球科学版),2012,42(6):1880—1888.
[24]郭强,田慧,吴有方,等.甘肃省及其周边地区土壤六氯苯污染特征[J].中国环境科学,2013,33(3):455—46.
[25]李军,张干,祁士华,等.珠江三角洲土壤中氯丹的残留特征[J].土壤学报,2007,44(6):1058—1062.
[26]孟晶,王铁宇,王佩,等.环河流域土壤中全氟化合物的空间分布及组成特征[J].环境科学,2013,34(8):3188—3194.
[27]Li K,Fu S,Yang Z Z,et al.Composition,distribution and characterization of polybrominated diphenyl ethers(PBDEs)in the soil in Taiyuan,China[J].Environmental Contamination and Toxicology,2008,81(6):588-593.
[28]潘波,施治,何新春,等.天津地区鱼塘中的HSHs残留[J].农业环境科学学报,2004,23(3):368—371.
[29]曹启民,王华,张黎明.中国持久性有机污染物污染现状及治理技术进展[J].农业资源与环境科学,2006,22(2):361—365.
[30]Wong M H,Leung A O W,Chan J K Y,et al.Are view on the usage of POP pesticidesin China,with emphasison DDT loadingsin human milk[J].Chemo sphere,2005,60(6):740-752.
[31]李冬梅,李建科,史志诚.持久性有机污染物的毒理学危害及其环境治理[A].毒理学史研究文集[C].西北大学,2007,7:2—9.
[32]Yuan D,Yang D,Wade T L,Qian Y.Status of persistent organic pollutants in the sediment from several estuaries in China[J].Environmental Pollution,2001,114:101-111.
[33]陈华林.沉积物对有机污染物的不可逆吸附行为[D].浙江大学,2003,5.
[34]Liu G Q,Yu L L,Li J,et al.PAHs in soils and estimated air soil exchange in the Pearl River Delta,South China[J].Environmental Monitoring and Assessment,2011,173(1-4):861-870.
[35]Vlckova K,Hofman J.A comparison of POPs bioaccumulation in Eisenia fetida in natural and artificial soils and the effects of aging[J].Environmental Pollution,2012,160:49-56.
[36]薛南冬,李发生,等.持久性有机污染物(POPs)污染场地风险控制与环境修复[M].北京:科学出版社,2011.
[37]Zabel E W,Walker M K,Homung M W,etal.Interactions of Polychlorinated Dibenzop-dioxin,Dibenzofuran,and Biphenyl Congeners for Producing Rainbow Trout Early Life Stage Mortality[J].Toxicology and Applied Pharmacology,1995,134(2):204-213.
[38]Muller C E,De Silva A O,Small J,et al.Biomagnification of perfluorinated compounds in a remote terrestrial food chain:Lichen-caribou-wolf[J].Environmental Science&Technology,2011.45(20):8665-8673.
[39]Liu Jia ying,Li Jing guang,Zhao Yun feng,etal.The occurrence of perfluorinated alkyl compounds in human milk from different regions of China[J].Environ International,2010,36(5):433-438.
[40]聂海峰,赵传冬,刘应汉,等.松花江流域河流沉积物中多氯联苯的分布、来源及风险评价[J].环境科学,2012,33(10):3434—3442.
[41]施召才.多氯联苯对男性生殖影响的研究[D].华南理工大学,2013.
[42]Haitao Shen,Gangqiang Ding,Yongning Wu,Guoshao Pan,Xiaoping Zhou,Jianlong Han,Jingguang Li,Sheng Wen.Polychlorinated dibenzo-p-dioxins/furans(PCDD/Fs),polychlorinated biphenyls(PCBs),and polybrominated diphenyl ethers(PBDEs)in breast milk from Zhejiang,China[J].Environment International.2012,42:84-90.
[43]黄莉,黄韧,冯媛瑜,等.2,3,7,8一四氯苯并二(?)英(TCDD)短期染毒可造成着床前胚胎丢失并伴随雌性生殖器官中毒物相关蛋白的诱导表达[J].生态毒理学报,2010,05(3):334—342.
[2]李扬,马运,黄启飞等.我国持久性有机污染物管理策略研究[J].环境科学与技术,2011,34(7):200-205.
[3]Zhang K,Zhang B Z,Li S M,et al.Regional dynamics of persistent organic pollutants(POPs)in the Pearl River Delta,China:Implications and perspectives[J].Environmental Pollution,2011,159(10):2301-2309.
[4]余刚,黄俊.持久性有机污染物知识100问[M].北京:中国环境科学出版社,2005.
[5]王亚鞯,蔡亚岐,江桂斌.斯德哥尔摩公约新增持久性有机污染物的一些研究进展[J].中国科学.化学,2010,40(2):99—123.
[6]余刚,牛军峰,黄俊,等.持久性有机污染物——新的全球性环境问题[M].北京:科学出版社,2005.
[7]Bao L J,Keith A M,Shane A S,et al.China's water pollution by persistent organic pollutants[J].Environmental Pollution,2012,163:100-108.
[8]马万里,刘丽艳,齐虹,等.松花江流域冰封期水体中多环芳烃的污染特征研究[J].环境科学,2012,33(12):4420-4425.
[9]Li G C,Xia X H,Wang R,et al.Pollution of polycyclic aromatic hydrocarbons(PAHs)in middle and lower reaches of the Yellow River[J].Environmental Science,2006,27(9):1738-1743.
[10]李秀丽,赖子尼,穆三妞,等.珠江入海口表层沉积物中多氯联苯残留与风险评价[J].生态环境学报,2012,21(12):135-140.
[11]冯承莲,夏星辉,周追,等.长江武汉段水体中多环芳烃的分布及来源分析[J].环境科学学报,2007,27(11):1900—1908.
[12]康跃惠,刘培斌,王子健,等.北京官厅水库—永定河水系水体中持久性有机氯农药污染[J].湖泊科学,2003,15(2):125—132.
[13]张伟玲,张干,祁士华,等.西藏错鄂湖和羊卓雍湖水体及沉积物中有机氯农药的初步研究[J].地球化学,2003,32(4):363—367.
[14]胡国成,郑海,张丽娟,等.珠江三角洲土壤中全氟化合物污染特征研究[J].中国环境科学,2013,33(S1):37-42.
[15]陈燕燕,尹颖,王晓蓉等.太湖表层沉积物中PAHs和PCBs的分布及风险评价[J].中国环境科学,2009,29(2):118—124.
[16]林田,马传良,王丽芳,等.滇池沉积物中多氯联苯和有机氯农药的残留特征与风险评估[J].地球与环境,2014,42(5):625—630.
[17]Guo Jian yang,Wu Feng chang,Liao Hai qing,et al.Sedimentary record of polycyclic aromatic hydrocarbons and DDTs in Dianchi Lake,an urban lake in Southwest China[J].Environmental Science and Pollution Research,2013,20(8):5471-5480.
[18]张帆,余应新,张东平,等.溴系阻燃剂在环境及人体中的存在和代谢转化[J].化学进展,2009,21(6):1364-1372.
[19]胡吉成.北京市大气中涣代阻燃刊环境行为的研究[M].中央民族大学,2010.
[20]Cooney C M.Detecting a new PCB in Chicago air[J].EnvironSciTechnol,2009,43(1):4-4.
[21]戴朝霞,陈振翔,王格慧,等.典型城市大气颗粒物中多环芳烃的污染研究[J].环境科学与技术,2006,2.
[22]Meijer S N,Ockenden W A,Sweetman A,et al.Global distribution and budget of PCBs and HCB in background surface soils:Implications for sources and environmental processes[J].Environmental Science&Technology,2003,37(4):667-672.
[23]崔嵩,杨萌,李一凡.不同土壤类型多氯联苯土壤残留特征变化分析[J].吉林大学学报(地球科学版),2012,42(6):1880—1888.
[24]郭强,田慧,吴有方,等.甘肃省及其周边地区土壤六氯苯污染特征[J].中国环境科学,2013,33(3):455—46.
[25]李军,张干,祁士华,等.珠江三角洲土壤中氯丹的残留特征[J].土壤学报,2007,44(6):1058—1062.
[26]孟晶,王铁宇,王佩,等.环河流域土壤中全氟化合物的空间分布及组成特征[J].环境科学,2013,34(8):3188—3194.
[27]Li K,Fu S,Yang Z Z,et al.Composition,distribution and characterization of polybrominated diphenyl ethers(PBDEs)in the soil in Taiyuan,China[J].Environmental Contamination and Toxicology,2008,81(6):588-593.
[28]潘波,施治,何新春,等.天津地区鱼塘中的HSHs残留[J].农业环境科学学报,2004,23(3):368—371.
[29]曹启民,王华,张黎明.中国持久性有机污染物污染现状及治理技术进展[J].农业资源与环境科学,2006,22(2):361—365.
[30]Wong M H,Leung A O W,Chan J K Y,et al.Are view on the usage of POP pesticidesin China,with emphasison DDT loadingsin human milk[J].Chemo sphere,2005,60(6):740-752.
[31]李冬梅,李建科,史志诚.持久性有机污染物的毒理学危害及其环境治理[A].毒理学史研究文集[C].西北大学,2007,7:2—9.
[32]Yuan D,Yang D,Wade T L,Qian Y.Status of persistent organic pollutants in the sediment from several estuaries in China[J].Environmental Pollution,2001,114:101-111.
[33]陈华林.沉积物对有机污染物的不可逆吸附行为[D].浙江大学,2003,5.
[34]Liu G Q,Yu L L,Li J,et al.PAHs in soils and estimated air soil exchange in the Pearl River Delta,South China[J].Environmental Monitoring and Assessment,2011,173(1-4):861-870.
[35]Vlckova K,Hofman J.A comparison of POPs bioaccumulation in Eisenia fetida in natural and artificial soils and the effects of aging[J].Environmental Pollution,2012,160:49-56.
[36]薛南冬,李发生,等.持久性有机污染物(POPs)污染场地风险控制与环境修复[M].北京:科学出版社,2011.
[37]Zabel E W,Walker M K,Homung M W,etal.Interactions of Polychlorinated Dibenzop-dioxin,Dibenzofuran,and Biphenyl Congeners for Producing Rainbow Trout Early Life Stage Mortality[J].Toxicology and Applied Pharmacology,1995,134(2):204-213.
[38]Muller C E,De Silva A O,Small J,et al.Biomagnification of perfluorinated compounds in a remote terrestrial food chain:Lichen-caribou-wolf[J].Environmental Science&Technology,2011.45(20):8665-8673.
[39]Liu Jia ying,Li Jing guang,Zhao Yun feng,etal.The occurrence of perfluorinated alkyl compounds in human milk from different regions of China[J].Environ International,2010,36(5):433-438.
[40]聂海峰,赵传冬,刘应汉,等.松花江流域河流沉积物中多氯联苯的分布、来源及风险评价[J].环境科学,2012,33(10):3434—3442.
[41]施召才.多氯联苯对男性生殖影响的研究[D].华南理工大学,2013.
[42]Haitao Shen,Gangqiang Ding,Yongning Wu,Guoshao Pan,Xiaoping Zhou,Jianlong Han,Jingguang Li,Sheng Wen.Polychlorinated dibenzo-p-dioxins/furans(PCDD/Fs),polychlorinated biphenyls(PCBs),and polybrominated diphenyl ethers(PBDEs)in breast milk from Zhejiang,China[J].Environment International.2012,42:84-90.
[43]黄莉,黄韧,冯媛瑜,等.2,3,7,8一四氯苯并二(?)英(TCDD)短期染毒可造成着床前胚胎丢失并伴随雌性生殖器官中毒物相关蛋白的诱导表达[J].生态毒理学报,2010,05(3):334—342.