用户名: 密码: 验证码:
负载型阳极板对PAM模拟废水的处理研究
详细信息    查看全文 | 推荐本文 |
  • 英文篇名:Effects of Supported Anode Plate on the Treatment of PAM Simulative Wastewater
  • 作者:舒帮云 ; 马伶俐 ; 易啸 ; 吴锋 ; 陈小军 ; 丁友智 ; 罗玉琳
  • 英文作者:Shu Bangyun;Ma Lingli;Yi Xiao;Wu Feng;Chen Xiaojun;Ding Youzhi;Luo Yulin;Sichuan National Inspection and Testing Co., Ltd.;Chongqing Ecological Environment Monitoring Center;
  • 关键词:三维电极 ; 阳极板 ; 聚丙烯酰胺
  • 英文关键词:three-dimensional electrode;;anode plate;;polyacrylamide
  • 中文刊名:广东化工
  • 英文刊名:Guangdong Chemical Industry
  • 机构:四川国检检测有限责任公司;重庆市生态环境监测中心;
  • 出版日期:2019-07-30
  • 出版单位:广东化工
  • 年:2019
  • 期:14
  • 语种:中文;
  • 页:153-154+162
  • 页数:3
  • CN:44-1238/TQ
  • ISSN:1007-1865
  • 分类号:X703
摘要
采用三相三维电极反应器处理PAM模拟废水,重点考察了不同负载型阳极板对PAM模拟废水处理效果、强氧化性物质产生以及电解能耗的影响。研究结果表明,当以Ti/SnSbCo作阳极时,CODcr去除率最高,为32.0%;电催化活性最强,产生强氧化性物质量最多,对有机物能够有效地降解去除。此外,采用Ti/SnSbCo作阳极对模拟废水进行处理,电解能耗最低,当CODcr去除率为15%时,其电解能耗为12.1kw·h/m3,较Ti作阳极板时节省能耗13.47 kw·h/m3。
        The PAM simulative wastewater was electrolytically treated by a three-phase three-dimensional electrode reactor. Particular attention was paid on the comparison of treatment efficiency, production of strong oxidizing substance and electrolysis energy consumption of different loaded anode plate in the system. The results verified when using Ti/SnSbCo as the anode, CODcr removal efficiency is up to32.0 %, Theelectrocatalytic activity is the strongest, generation of oxidizing substance is the most and the organic matter can be effectively degraded and removed. Moreover, the energy consumption is the lowest using Ti/SnSbCo as anode to treat simulated wastewater, when the CODcr removal efficiency was 15 %, the electrolysis energy consumption was 13.47 kw·h/m3 lower than thatusing Ti as anode.
引文
[1]Gregory K B,Vidic R D,Dzombak D A.Water Management Challenges Associated with the Production of Shale gas by Hydraulic Fracturing[J].Elements,2011,7(3):181-186.
    [2]杨德敏,袁建梅,夏宏,等.页岩气开发过程中存在的环境问题及对策[J].油气田环境保护,2013,23(2):68-69.
    [3]叶春松,郭京骁,周为,等.页岩气压裂返排液处理技术的研究进展[J].化工环保,2015,35(01):21-26.
    [4]唐颖,张金川,张琴,等.页岩气井水力压裂技术及其应用分析[J].开发工程,2010,30(10):33-38.
    [5]李辉,杨志刚,何飞,等.陆相页岩气压裂返排液循环利用技术概述[J].油气田环境保护,2014,24(01):24-26.
    [6]付茜,彭其勇.页岩气压裂返排液对环境的影响及思考[J].油气田环境保护,2015,25(03):60-63.
    [7]Shaffer D L,Arias Chavez L H,Bensasson M,et al.Desalination and reuse of high-salinity shale gas produced water:drivers,technologies,and future directions[J].Environmental Science&Technology,2013,47(17):9569-83.
    [8]Backhurst J R, Conclson J M, Goodridge F, et al. A proliminaryinvestignation of fluidized bed electrodes[J].Electrochem,1969,116(11):1600-1607.
    [9]张鹏娟,买文宁,赵敏,等.三维电极法深度处理维生素生产废水[J].环境工程学报,2013,7(3):897-902.
    [10]熊英健,范娟,朱锡海.三维电极电化学水处理技术研究现状及方向[J].工业水处理,1998,18(1):5-8.
    [11]陈武,李凡修,梅平,等.废水处理的电化学方法研究进展[J].湖北化工,2001,3(1):10-12.
    [12]陈卫国,朱锡海.电催化产生H2O2和·OH及去除废水中有机污染物的应用[J].中国环境科学,1998,18(02):53-55.
    [13]Fockedey E,Van L A.Coupling of anodic and cathodic reactions for phenol electro-oxidation using three-dimensional electrodes[J]. Water Research,2002,36(16):4169.
    [14]张翼,周新新,韩大匡,等.稀土La掺杂SnSb复合涂层Ti基电极的制备及催化性能[J].材料保护,2010,43(06):9-12.
    [15]Slavik E,Galessi R,Rapisardi A,et al.Wet oxidation as an advanced and sustainable technology for sludge treatment and management:results from research activities and industrial-scale experiences[J].Drying Technology,2015,33(11):1309-1317.
    [16]吕贵芬,张珠宝,吴丁财,等.三维电极法降解苯酚废水中·OH的测定及其影响因素研究[J].中山大学学报:自然科学版,2009,48(5):78-81.

© 2004-2018 中国地质图书馆版权所有 京ICP备05064691号 京公网安备11010802017129号

地址:北京市海淀区学院路29号 邮编:100083

电话:办公室:(+86 10)66554848;文献借阅、咨询服务、科技查新:66554700