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氢自养反硝化细菌对纳米铁沉降性能的影响
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  • 英文篇名:Effect of hydrogenotrophic bacteria on sedimentation of nanoscale zero-valent iron
  • 作者:刘瑞阳 ; 岳俊杰 ; 韩温诺 ; 安毅
  • 英文作者:Liu Ruiyang;Yue Junjie;Han Wennuo;An Yi;School of Environmental Science and Safety Engineering,Tianjin University of Technology;Innovative Team of Monitoring and Precaution for Cropland Environment,Institute of Agro-Environmental Protection,Ministry of Agriculture;
  • 关键词:纳米零价铁 ; 氢自养反硝化细菌 ; 腐殖酸 ; 沉降性
  • 英文关键词:nanoscale zero-valent iron;;hydrogenotrophic bacteria;;humic acid;;sedimentation
  • 中文刊名:工业水处理
  • 英文刊名:Industrial Water Treatment
  • 机构:天津理工大学环境科学与安全工程学院;农业部环境保护科研监测所产地环境监测与预警创新团队;
  • 出版日期:2019-10-20
  • 出版单位:工业水处理
  • 年:2019
  • 期:10
  • 基金:国家自然科学基金项目(41573107)
  • 语种:中文;
  • 页:49-52
  • 页数:4
  • CN:12-1087/X
  • ISSN:1005-829X
  • 分类号:X523
摘要
通过静态沉降实验,考察了氢自养反硝化细菌(HTB)在不同水质条件下对纳米零价铁(nZVI)沉降性能的影响。结果表明:当体系中腐殖酸(HA)质量浓度为10 mg/L时,1/3HTB对nZVI沉降性的抑制作用最明显。K+和Ca~(2+)对nZVI的沉降有促进作用;K+浓度为3、6 mmol/L时,HTB对nZVI的沉降性有抑制作用,在不同浓度Ca~(2+)条件下,HTB对nZVI的沉降性均有促进作用,可加速nZVI的沉降。
        Static sedimentation experiments were conducted to investigate the effects of hydrogenotrophic bacteria(HTB) on the sedimentation of nZVI under different water quality conditions. The experimental results showed that when the concentration of HA in the system was 10 mg/L,1/3 HTB had the most obvious inhibitory effect on the sedimentation of nZVI. Both K+and Ca~(2+)promoted the sedimentation of nZVI. When the concentration of K+in the system was 3 or 6 mmol/L, HTB inhibited the sedimentation of nZVI. However, when Ca~(2+)was present in the system, HTB accelerated the sedimentation of nZVI.
引文
[1] Lefevre E,Bossa N,Wiesner M R,et al. A review of the environmental implications of in situ remediation by nanoscale zero valent iron(n ZVI):Behavior,transport and impacts on microbial communities[J]. Science of the Total Environment,2016,565:889-901.
    [2] Dong Haoran,Zhao Feng,He Qi,et al. Physicochemical transformation of carboxymethyl cellulose-coated zero-valent iron nanoparticles(nZVI)in simulated groundwater under anaerobic conditions[J]. Separation and Purification Technology,2017,175:376-383.
    [3] Lin S,Wiesner M R. Deposition of aggregated nanoparticles:A theoretical and experimental study on the effect of aggregation state on the affinity between nanoparticles and a collector surface[J]. Environmental Science&Technology,2012,46(24):13270-13277.
    [4] Adamczyk Z,Siwek B,Zembala M,et al. Kinetics of localized adsorption of colloid particles[J]. Advances in Colloid and Interface Science,1994,48:151-280.
    [5] Han Peng,Zhou Dan,Tong Meiping,et al. Effect of bacteria on the transport and deposition of multi-walled carbon nanotubes in saturated porous media[J]. Environmental Pollution,2016,213:895-903.
    [6] Jung B,O’carroll D,Sleep B. The influence of humic acid and clay content on the transport of polymer-coated iron nanoparticles through sand[J]. Science of the Total Environment,2014,496:155-164.
    [7] Wang Wei,Jin Zhaohui,Li Tielong,et al. Preparation of spherical iron nanoclusters in ethanol-water solution for nitrate removal[J].Chemosphere,2006,65(8):1396-1404.
    [8] An Yi,Dong Qi,Zhang Keqiang. Bioinhibitory effect of hydrogenotrophic bacteria on nitrate reduction by nanoscale zero-valent iron[J].Chemosphere,2014,103:86-91.
    [9] Shin K H,Cha D K. Microbial reduction of nitrate in the presence of nanoscale zero-valent iron[J]. Chemosphere,2008,72(2):257-262.
    [10] Dong H,Ahmad K,Zeng G,et al. Influence of fulvic acid on the colloidal stability and reactivity of nanoscale zero-valent iron[J]. Environmental Pollution,2016,211:363-369.
    [11] Ouyang Kai,Yu Xiaoying,Zhu Yunlin,et al. Effects of humic acid on the interactions between zinc oxide nanoparticles and bacterial biofilms[J]. Environmental Pollution,2017,231:1104-1111.
    [12] Esfahani A R,Firouzi A F,Sayyad G,et al. Transport and retention of polymer-stabilized zero-valent iron nanoparticles in saturated porous media:Effects of initial particle concentration and ionic strength[J]. Journal of Industrial and Engineering Chemistry,2014,20(5):2671-2679.

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