川东—渝北地区石炭系白云岩成因与成岩系统研究
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摘要
白云岩的成因问题是碳酸盐岩岩石学中最复杂、争论时间最久、最难解决的岩石学难题之一,成岩系统研究是成岩作用研究发展进程中与盆地动力学相结合的前沿研究领域。川东―渝北地区黄龙组碳酸盐岩在漫长的成岩历史中经历了准同生期孔隙水成岩系统、早成岩埋藏期压释卤水成岩系统、古表生期大气水成岩系统和再埋藏中―晚成岩期温压水成岩系统的复杂改造,最终形成了以晶粒白云岩、颗粒白云岩和白云质岩溶角砾岩为主的碳酸盐岩储层,可见研究该地区白云岩成因和成岩系统两大基础地质问题是评价黄龙组碳酸盐岩储层形成机理的关键,因此,对黄龙组储层的白云岩成因和成岩系统开展研究,不仅具有重要理论意义,更具实践意义。
本论文在总结国内外相关研究最新成果的基础上,结合区域地质背景,采用岩矿鉴定技术以及碳氧锶稳定同位素、微量元素、稀土元素和包裹体等测试手段,对黄龙组白云岩成因和成岩系统及其与储层的发育关系进行了系统深入的研究,取得以下几点主要成果和新认识:
1.通过野外剖面、岩心观察和室内岩矿分析结果,识别出微晶白云岩、粉-细晶白云岩、颗粒白云岩、白云质岩溶角砾岩、淡水白云石和热液白云岩等白云岩(石)类型,按照结构―成因分类,将其划分为准同生期白云岩、早成岩期埋藏白云岩、古表生期溶蚀白云岩和淡水白云石胶结物,以及再埋藏期的热液白云岩四种成因类型,不同期次和成因的白云岩(石),具有随着成岩强度加强,白云石有序度增高和MgCO3/CaCO3比值逼近1的演化趋势。
2.层序―岩相古地理特征分析认为,黄龙组层序低位体系域时发育的萨勃哈、海侵体系域时间歇性海退期在局限区域形成的干旱蒸发环境提供了大量的封存地层卤水,为早成岩阶段的埋藏白云岩化作用提供了流体来源物质条件,海侵体系域发育的障壁滩和滨外粒屑滩相是早成岩期埋藏白云岩化作用最活跃区域,也是最有利储层发育的相带。
3.碳、氧同位素地球化学特征分析结果,表明成岩期埋藏白云岩化流体来源于早期萨勃哈环境封存的地层卤水,古表生期的岩溶作用和淡水白云石和方解石的成因与大气水溶蚀有关,而再埋藏成岩期的异形白云石为深源热液溶蚀白云质基质岩的沉淀物。
4.锶同位素地球化学特征分析结果,进一步证明了成岩期埋藏白云岩流体来源于黄龙组一段的海源地层卤水,岩溶岩的溶蚀与沉淀于孔洞缝的淡水白云石和方解石胶结物的流体来源于古表生期的大气淡水,而异形白云石是深部热液流体参与成岩作用的产物。
5.稀土元素地球化学特征分析结果,表明准同生期和成岩期白云岩化过程中强烈的REE迁移贫化过程,是在性质相似的成岩流体中进行的,即成岩埋藏白云岩流体来源于准同生期封存在地层中的卤水,岩溶岩的溶蚀与淡水白云石和方解石胶结物的沉淀,形成于弱氧化的低温大气水流体中,而异形白云石的稀土元素特征也反映其为再埋藏期热液溶蚀基质白云岩后沉淀的热水矿物。
6.根据不种成因类型的白云岩(石)各项地球化学特征及其所反映的成岩流体性质,按“水文体制”与相对应的成岩作用方式和相应的产物与组合特征,将黄龙组白云岩(石)的成岩演化历史划分为四个流体来源、性质、水―岩石相互作用过程各不相同,但连续演化的成岩系统,即准同生期孔隙卤水成岩系统、早成岩期压释地层卤水成岩系统、古表生期下渗大气水成岩系统和再埋藏期深部温压水成岩系统。
7.讨论了成岩体系与储层发育的关系,认为与储层发育关系最密切的是早成岩阶段压释卤水成岩系统的埋藏白云岩化作用、古表生期下渗大气水成岩系统的岩溶作用和再埋藏期中、晚成岩阶段的构造破裂作用。
Dolomite genesis problem is one of the most complex,disputing and difficultly resolving carbonate petrology difficulty,and diagenesis system study is a new frontier field combined with Sedimentary Basin Dynamics during developing diagenesis study. By the complex reconstruction of the penecontemporaneous pore water diagenetic stage,atmospheric water diagenesis system at ancient epigenenesis,early diagenetic burial stage of compaction brine diagenesis system and the middle to late re-buried temperature and pressure water diagenetic stage in eastern Sichuan-northern Chongqing area,carbonate of Huanglong Formation ultimately form carbonate reservoir which included three main rock types of grain dolomite ,crystalline doloston and corrosion-brecciated of karst rock. Dolomite genesis and Hydrological system are the key of evaluating carbonate reservoir of Huanglong Formation. So,the study of dolomite genesis and diagenesis system of Huanglong Formation reservoir not only important for theory significance, but also for practice significance.
Based on the new conclusion of inland and overseas , and combined with the palaeogeographical setting of the study area,used instrumentations of lithology-mineral identification techniques;Carbon,Oxygen ,strontium stable isotopes;trace elements;rare earth elements and inclusion,by study of Dolomite genesis and diagenesis system and there relations with reservoir of Huanglong Formation ,the may conclusions and new recognitions as follows:
1. Through comprehensive analysis of field section, well core description and lithology-mineral in house,dolomite styles of dolomicrite,crystal powder-fine dolomite, grain dolomite , corrosion-brecciated of karst rock , the fresh water dolomization , hydrothermal dolomization have been recognized. By classify with composition-genesis,the four models of dolomization have been set up:the penecontemporaneous dolomization,the burial diagenetic dolomization , the fresh water dolomization of epidiagenesis and hydrothermal dolomization of late diagenetic stage. Dolomite with different stages and genesis have the evolutionary trend of strengthen by diagenesis intensity,dolomite degree of order get higher,MgCO3/CaCO3 ratio arise trend of 1.
2. Through the characteristics of sequence-based lithofacies and paleogeography,sabkha facie which developed on period of The low system tract sequence,the evaporation environment which developed on period of episodic regression stage of transgression system tract in limitate area,and layer brine water which seal up in this environment offer fluid original source material condition for early diagenetic stage burial dolomitization . The barrier grain beach and offshore grain beach in TST period are the most active area of the early burial diagenetic,And are thought the most favourite reservoir facies.
3. Based on the characteristics of Carbon,Oxygen stable isotopes, the diagenetic burial dolomitizing fluids came from burial brine water of early stage sabkha environment,the genesis of karstification of epidiagenetic stage and limnic-dolomite and limnic-Calcite have related with atmospheric water corrosion,hydrothermal dolomite of reburial period is the precipitate of deep hydrothermal fluid corroded dolomitic matrix rock.
4. By the synthetical analysis of geochemical characteristics of Sr isotope,further demonstrate that the diagenetic burial dolomitizing fluids came from sea origin brine water of Huanglong FormationⅠ, fluids of karstification of karst rocks and the cement of limnic-dolomite and limnic-Calcite came from atmospheric water of epidiagenetic stage,and hydrothermal dolomite is the result of deep hydrothermal fluid participated in diagenesis.
5. By the synthetical analysis of geochemical characteristics of rare earth elements,the conclusion that the removing of the REE at dolomitization process strongly in the penecontemporaneous stage and diagenetic burial stage,the diagenetic burial dolomitizing fluids came from brine water of penecontemporaneous stage,karstification of karst rocks and the cement of limnic-dolomite and limnic-Calcite take shape from weak oxygenated low temperature atmospheric water fluids. Rare earth elements characteristics of hydrothermal dolomite reflected it’s the hydrotherm mineral of hydrothermal fluid corroded matrix dolomite rock on reburial period.
6. According to geochemical behavior and diagenetic fluid property of different genetic types dolomite,though“Hydrological system”and the manner of diagenesis,researching of corresponding product of geology,combination,evolution stage of diagenesis in Huanglong Formation are divided into four fuild origin,property,water-rock interaction process,the effect of them to the reservoir development are also different. So the diagenesis systems and manner of diagenesis,are mainly as follows:the penecontemporaneous stage pore water diagenesis system;early diagenetic burial stage of compaction brine diagenesis system;ancient epigenenesis atmospheric water diagenesis system at and re-buried deep temperature and pressure water diagenetic stage.
7. Discussed the relations of the diagenesis systems and reservoir development, which related to the reservoir development closely,are mainly as follows:the role of burial dolomitization of compaction brine diagenesis system at early diagenetic stage ; the karstification of atmospheric water diagenesis system at ancient epigenenesis; the role of tectonic disruption at the middle to late re-buried diagenetic stage.
本论文在总结国内外相关研究最新成果的基础上,结合区域地质背景,采用岩矿鉴定技术以及碳氧锶稳定同位素、微量元素、稀土元素和包裹体等测试手段,对黄龙组白云岩成因和成岩系统及其与储层的发育关系进行了系统深入的研究,取得以下几点主要成果和新认识:
1.通过野外剖面、岩心观察和室内岩矿分析结果,识别出微晶白云岩、粉-细晶白云岩、颗粒白云岩、白云质岩溶角砾岩、淡水白云石和热液白云岩等白云岩(石)类型,按照结构―成因分类,将其划分为准同生期白云岩、早成岩期埋藏白云岩、古表生期溶蚀白云岩和淡水白云石胶结物,以及再埋藏期的热液白云岩四种成因类型,不同期次和成因的白云岩(石),具有随着成岩强度加强,白云石有序度增高和MgCO3/CaCO3比值逼近1的演化趋势。
2.层序―岩相古地理特征分析认为,黄龙组层序低位体系域时发育的萨勃哈、海侵体系域时间歇性海退期在局限区域形成的干旱蒸发环境提供了大量的封存地层卤水,为早成岩阶段的埋藏白云岩化作用提供了流体来源物质条件,海侵体系域发育的障壁滩和滨外粒屑滩相是早成岩期埋藏白云岩化作用最活跃区域,也是最有利储层发育的相带。
3.碳、氧同位素地球化学特征分析结果,表明成岩期埋藏白云岩化流体来源于早期萨勃哈环境封存的地层卤水,古表生期的岩溶作用和淡水白云石和方解石的成因与大气水溶蚀有关,而再埋藏成岩期的异形白云石为深源热液溶蚀白云质基质岩的沉淀物。
4.锶同位素地球化学特征分析结果,进一步证明了成岩期埋藏白云岩流体来源于黄龙组一段的海源地层卤水,岩溶岩的溶蚀与沉淀于孔洞缝的淡水白云石和方解石胶结物的流体来源于古表生期的大气淡水,而异形白云石是深部热液流体参与成岩作用的产物。
5.稀土元素地球化学特征分析结果,表明准同生期和成岩期白云岩化过程中强烈的REE迁移贫化过程,是在性质相似的成岩流体中进行的,即成岩埋藏白云岩流体来源于准同生期封存在地层中的卤水,岩溶岩的溶蚀与淡水白云石和方解石胶结物的沉淀,形成于弱氧化的低温大气水流体中,而异形白云石的稀土元素特征也反映其为再埋藏期热液溶蚀基质白云岩后沉淀的热水矿物。
6.根据不种成因类型的白云岩(石)各项地球化学特征及其所反映的成岩流体性质,按“水文体制”与相对应的成岩作用方式和相应的产物与组合特征,将黄龙组白云岩(石)的成岩演化历史划分为四个流体来源、性质、水―岩石相互作用过程各不相同,但连续演化的成岩系统,即准同生期孔隙卤水成岩系统、早成岩期压释地层卤水成岩系统、古表生期下渗大气水成岩系统和再埋藏期深部温压水成岩系统。
7.讨论了成岩体系与储层发育的关系,认为与储层发育关系最密切的是早成岩阶段压释卤水成岩系统的埋藏白云岩化作用、古表生期下渗大气水成岩系统的岩溶作用和再埋藏期中、晚成岩阶段的构造破裂作用。
Dolomite genesis problem is one of the most complex,disputing and difficultly resolving carbonate petrology difficulty,and diagenesis system study is a new frontier field combined with Sedimentary Basin Dynamics during developing diagenesis study. By the complex reconstruction of the penecontemporaneous pore water diagenetic stage,atmospheric water diagenesis system at ancient epigenenesis,early diagenetic burial stage of compaction brine diagenesis system and the middle to late re-buried temperature and pressure water diagenetic stage in eastern Sichuan-northern Chongqing area,carbonate of Huanglong Formation ultimately form carbonate reservoir which included three main rock types of grain dolomite ,crystalline doloston and corrosion-brecciated of karst rock. Dolomite genesis and Hydrological system are the key of evaluating carbonate reservoir of Huanglong Formation. So,the study of dolomite genesis and diagenesis system of Huanglong Formation reservoir not only important for theory significance, but also for practice significance.
Based on the new conclusion of inland and overseas , and combined with the palaeogeographical setting of the study area,used instrumentations of lithology-mineral identification techniques;Carbon,Oxygen ,strontium stable isotopes;trace elements;rare earth elements and inclusion,by study of Dolomite genesis and diagenesis system and there relations with reservoir of Huanglong Formation ,the may conclusions and new recognitions as follows:
1. Through comprehensive analysis of field section, well core description and lithology-mineral in house,dolomite styles of dolomicrite,crystal powder-fine dolomite, grain dolomite , corrosion-brecciated of karst rock , the fresh water dolomization , hydrothermal dolomization have been recognized. By classify with composition-genesis,the four models of dolomization have been set up:the penecontemporaneous dolomization,the burial diagenetic dolomization , the fresh water dolomization of epidiagenesis and hydrothermal dolomization of late diagenetic stage. Dolomite with different stages and genesis have the evolutionary trend of strengthen by diagenesis intensity,dolomite degree of order get higher,MgCO3/CaCO3 ratio arise trend of 1.
2. Through the characteristics of sequence-based lithofacies and paleogeography,sabkha facie which developed on period of The low system tract sequence,the evaporation environment which developed on period of episodic regression stage of transgression system tract in limitate area,and layer brine water which seal up in this environment offer fluid original source material condition for early diagenetic stage burial dolomitization . The barrier grain beach and offshore grain beach in TST period are the most active area of the early burial diagenetic,And are thought the most favourite reservoir facies.
3. Based on the characteristics of Carbon,Oxygen stable isotopes, the diagenetic burial dolomitizing fluids came from burial brine water of early stage sabkha environment,the genesis of karstification of epidiagenetic stage and limnic-dolomite and limnic-Calcite have related with atmospheric water corrosion,hydrothermal dolomite of reburial period is the precipitate of deep hydrothermal fluid corroded dolomitic matrix rock.
4. By the synthetical analysis of geochemical characteristics of Sr isotope,further demonstrate that the diagenetic burial dolomitizing fluids came from sea origin brine water of Huanglong FormationⅠ, fluids of karstification of karst rocks and the cement of limnic-dolomite and limnic-Calcite came from atmospheric water of epidiagenetic stage,and hydrothermal dolomite is the result of deep hydrothermal fluid participated in diagenesis.
5. By the synthetical analysis of geochemical characteristics of rare earth elements,the conclusion that the removing of the REE at dolomitization process strongly in the penecontemporaneous stage and diagenetic burial stage,the diagenetic burial dolomitizing fluids came from brine water of penecontemporaneous stage,karstification of karst rocks and the cement of limnic-dolomite and limnic-Calcite take shape from weak oxygenated low temperature atmospheric water fluids. Rare earth elements characteristics of hydrothermal dolomite reflected it’s the hydrotherm mineral of hydrothermal fluid corroded matrix dolomite rock on reburial period.
6. According to geochemical behavior and diagenetic fluid property of different genetic types dolomite,though“Hydrological system”and the manner of diagenesis,researching of corresponding product of geology,combination,evolution stage of diagenesis in Huanglong Formation are divided into four fuild origin,property,water-rock interaction process,the effect of them to the reservoir development are also different. So the diagenesis systems and manner of diagenesis,are mainly as follows:the penecontemporaneous stage pore water diagenesis system;early diagenetic burial stage of compaction brine diagenesis system;ancient epigenenesis atmospheric water diagenesis system at and re-buried deep temperature and pressure water diagenetic stage.
7. Discussed the relations of the diagenesis systems and reservoir development, which related to the reservoir development closely,are mainly as follows:the role of burial dolomitization of compaction brine diagenesis system at early diagenetic stage ; the karstification of atmospheric water diagenesis system at ancient epigenenesis; the role of tectonic disruption at the middle to late re-buried diagenetic stage.
引文
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