春季境外生物质燃烧对东亚臭氧污染的影响
|
摘要
目的定量研究境外生物质燃烧对春季东亚地表臭氧浓度的影响。方法利用敏感性分析法与线性加权法,使用全球化学传输模式GEOS-Chem模拟春季全球不同地区生物质燃烧排放对东亚地表臭氧的贡献。结果春季全球生物质燃烧对东亚地表臭氧贡献在1×10~(-9)～5×10~(-9)(按体积计算)之间,其中75%是境外生物质燃烧的贡献。境外生物质燃烧对中国南部的影响比东亚其他区域更大,可达3×10~(-9)。在所有境外源区中,生物质燃烧对东亚地表臭氧影响最大的源区是非洲与东南亚。前者是中国东北部、中国北部、朝韩及日本地区的主要境外贡献区域。后者对中国南部的相对贡献最大。结论春季境外生物质燃烧对东亚地表臭氧的贡献具有一定的空间差异。境外生物质燃烧对东亚空气质量有重要影响。东亚地表臭氧污染治理需要世界各国及区域之间的良好合作。
Objective To study the impact of biomass burning emissions from foreign regions on surface ozone over East Asia in the spring. Methods Combining a sensitivity test and the linear weighting method, we simulated the individual contribution of biomass burning from different foreign regions in the world to surface ozone in East Asia with a global chemical transport model, GEOS-Chem. Results Biomass burning in the Spring of the world contributed 1×10~(-9)～5×10~(-9) to surface ozone in East Asia, in which, fire-induced ozone from foreign regions accounted for 75%. Fire-induced ozone from foreign regions contributed more to South China than to other regions in East Asia, reaching approximately 3×10~(-9). Among all the foreign regions,Southeast Asia and Africa were the largest contributors. Fire-induced ozone from Southeast Asia mainly influenced surface ozone in South China, while Africa imposed the largest foreign influences over Northeast China, North China, Korea, and Japan.The later had relatively large influences on South China. Conclusion The influence of biomass burning in foreign regions to springtime surface ozone in East Asia varies largely in space. Biomass burning in foreign regions can impact air quality in East Asia. Regional and international collaborations are needed for ozone pollution control in East Asia.
Objective To study the impact of biomass burning emissions from foreign regions on surface ozone over East Asia in the spring. Methods Combining a sensitivity test and the linear weighting method, we simulated the individual contribution of biomass burning from different foreign regions in the world to surface ozone in East Asia with a global chemical transport model, GEOS-Chem. Results Biomass burning in the Spring of the world contributed 1×10~(-9)～5×10~(-9) to surface ozone in East Asia, in which, fire-induced ozone from foreign regions accounted for 75%. Fire-induced ozone from foreign regions contributed more to South China than to other regions in East Asia, reaching approximately 3×10~(-9). Among all the foreign regions,Southeast Asia and Africa were the largest contributors. Fire-induced ozone from Southeast Asia mainly influenced surface ozone in South China, while Africa imposed the largest foreign influences over Northeast China, North China, Korea, and Japan.The later had relatively large influences on South China. Conclusion The influence of biomass burning in foreign regions to springtime surface ozone in East Asia varies largely in space. Biomass burning in foreign regions can impact air quality in East Asia. Regional and international collaborations are needed for ozone pollution control in East Asia.
引文
[1]LELIEVELD J,DENTENER F J.What Controls Tropospheric Ozone[J].Journal of Geophysical Research,2000,105:3531-3551.
[2]MCLINDEN C A,OLSEN S C,HANNEGAN B,et al.Stratospheric Ozone in 3-D Models:A Simple Chemistry and the Cross-tropopause Flux[J].Journal of Geophysical Research,2000,105:14653-14665.
[3]ZHANG Q,HE K B,HUO H.Cleaning China′s Air[J].Nature,2012,484:161-162.
[4]WANG T,XUE L,BRIMBLECOMBE P,et al.Ozone Pollution in China:A Review of Concentrations,Meteorological Influences,Chemical Precursors,and Effects[J].Science of the Total Environment,2017,575:1582-1596.
[5]CHANG K L,PETROPAVLOVSKIKH I,COOPER O R,et al.Regional Trend Analysis of Surface Ozone Observations from Monitoring Networks in Eastern North America,Europe and East Asia[J].Elementa:Science of the Anthropocene,2017,5:50-72.
[6]GAUDEL A,COOPER O,ANCELLET G,et al.Tropospheric Ozone Assessment Report:Present-day Distribution and Trends of Tropospheric Ozone Relevant to Climate and Global Atmospheric Chemistry Model Evaluation[J].Elementa:Science of the Anthropocene,2018,6:39.
[7]DING A,HUANG X,FU C.Air Pollution and Weather Interaction in East Asia[J].Oxford Research Encyclopedias-Environmental Science,2017,1:1-26.
[8]XU W,XU X,LIN M,et al.Long-term Trends of Surface Ozone and Its Influencing Factors at the Mt Waliguan GAW Station,China-Part 2:The Roles of Anthropogenic Emissions and Climate Variability[J].Atmospheric Chemistry and Physics,2018,18:773-798.
[9]SUN W,SHAO M,GRANIER C,et al.Long-Term Trends of Anthropogenic SO2,NOx,CO,and NMVOCs Emissions in China[J].Earth's Future,2018,6:1112-1133.
[10]ZHENG B,TONG D,LI M,et al.Trends in China's Anthropogenic Emissions Since 2010 as the Consequence of Clean Air Actions[J].Atmospheric Chemistry and Physics,2018,18:14095-14111.
[11]LU X,HONG J,ZHANG L,et al.Severe Surface Ozone Pollution in China:A Global Perspective[J].Environmental Science&Technology Letters,2018,5:487-494.
[12]SEKIYA T,SUDO K.Roles of Transport and Chemistry Processes in Global Ozone Change on Interannual and Multidecadal Time Scales[J].Journal of Geophysical Research,2014,119:4903-4921.
[13]DING A,FU C,YANG X,et al.Ozone and Fine Particle in the Western Yangtze River Delta:An Overview of 1Year Data at the SORPES Station[J].Atmospheric Chemistry and Physics,2013,13:5813-5830.
[14]JIANG Y,ZHAO T,LIU J,et al.Why Does Surface Ozone Peak before a Typhoon Landing in Southeast China[J].Atmospheric Chemistry and Physics,2015,15:13331-13338.
[15]ZHOU D,DING A,MAO H,et al.Impacts of the East Asian Monsoon on Lower Tropospheric Ozone over Coastal South China[J].Environmental Research Letters2013,8:044011.
[16]YANG Y,LIAO H,LI J.Impacts of the East Asian Summer Monsoon on Interannual Variations of Summertime Surface-layer Ozone Concentrations over China[J].Atmospheric Chemistry and Physics,2014,14:6867-6879.
[17]LI S,WANG T,HUANG X,et al.Impact of East Asian Summer Monsoon on Surface Ozone Pattern in China[J].Journal of Geophysical Research,2018,123:1401-1411.
[18]LIU H,JACOB D J,CHAN L Y,et al.Sources of Tropospheric Ozone Along the Asian Pacific Rim:An Analysis of Ozone Sonde Observations[J].Journal of Geophysical Research,2002,107:D21.
[19]FIORE A M,DENTENER F J,WILD O,et al.Multimodel Estimates of Intercontinental Source-receptor Relationships for Ozone Pollution[J].Journal of Geophysical Research,2009,114:D04301.
[20]DOHERTY R M.Ozone Pollution from Near and Far[J].Nature Geoscience,2015,8:664.
[21]HAN H,LIU J,YUAN H,et al.Impacts of Synoptic Weather Patterns and Their Persistency on Free Tropospheric Carbon Monoxide Concentrations and Outflow in Eastern China[J].Journal of Geophysical Research,2018,123:7024-7046.
[22]HAN H,LIU J,YUAN H,et al.Characteristics of Intercontinental Transport of Tropospheric Ozone from Africa to Asia[J].Atmospheric Chemistry and Physics,2018,18:4251-4276.
[23]ZHU Y,LIU J,WANG T,et al.The Impacts of Meteorology on the Seasonal and Interannual Variabilities of Ozone Transport from North America to East Asia[J].Journal of Geophysical Research,2017,122:10612-10636.
[24]YOSHITOMI M,WILD O,AKIMOTO H.Contributions of Regional and Intercontinental Transport to Surface Ozone in the Tokyo Area[J].Atmospheric Chemistry and Physics,2011,11:7583-7599.
[25]NAGASHIMA T,SUDO K,AKIMOTO H,et al.Long-term Change in the Source Contribution to Surface Ozone over Japan[J].Atmospheric Chemistry and Physics,2017,17:8231-8246.
[26]ZHANG L,JACOB D J,KOPACZ M,et al.Intercontinental Source Attribution of Ozone Pollution at Western U.S.Sites Using an Adjoint Method[J].Geophysical Research Letters,2009,36:L11810.
[27]COOPER O R,LANGFORD A O,PARRISH D D,et al.Challenges of a Lowered U.S.Ozone Standard,Science[J].2015,348:1096-1097.
[28]HUANG M,CARMICHAEL G R,PIERCE R B,et al.Impact of Intercontinental Pollution Transport on North American Ozone Air Pollution:An HTAP Phase 2Multi-model Study[J].Atmospheric Chemistry and Physics,2017,17:5721-5750.
[29]DENTENER F,KEATING T,AKIMOTO H.HTAP:Hemispheric Transport of Air Pollution 2010[M].United Nations:New York and Geneva,2010.
[30]NI R,LIN J,YAN Y,et al.Foreign and Domestic Contributions to Springtime Ozone Over China[J].Atmospheric Chemistry and Physics,2018,18:11447-11469.
[31]VAN der WERF G R,RANDERSON J T,GIGLIO L,et al.Global Fire Emissions Estimates during 1997-2016[J].Earth System Science Data,2017,9:697-720.
[32]DING A,FU C,YANG X,et al.Intense Atmospheric Pollution Modifies Weather:A Case of Mixed Biomass Burning with Fossil Fuel Combustion Pollution in Eastern China[J].Atmospheric Chemistry and Physics,2013,13:10545-10554.
[33]HUANG X,DING A,LIU L,et al.Effects of Aerosol-radiation Interaction on Precipitation during Biomass-burning Season in East China[J].Atmospheric Chemistry and Physics,2016,16:10063-10082.
[34]TANG H,LIU G,ZHU J,et al.Seasonal Variations in Surface Ozone as Influenced by Asian Summer Monsoon and Biomass Burning in Agricultural Fields of the Northern Yangtze River Delta[J].Atmospheric Research,2013,122:67-76.
[35]CHAN K.Biomass Burning Sources and Their Contributions to the Local Air Quality in Hong Kong[J].Science of The Total Environment,2017,596-597:212-221.
[36]DING K,LIU J,DING A,et al.Uplifting of Carbon Monoxide from Biomass Burning and Anthropogenic Sources to the Free Troposphere in East Asia[J].Atmospheric Chemistry and Physics,2015,15:2843-2866.
[37]BEY I,JACOB D J,YANTOSCA R M,et al.Global Modeling of Tropospheric Chemistry with Assimilated Meteorology:Model Description and Evaluation[J].Journal of Geophysical Research,2001,106:23073-23095.
[38]ZHANG L,JACOB D J,BOERSMA K F,et al.Transpacific Transport of Ozone Pollution and the Effect of Recent Asian Emission Increases on Air Quality in North America:An Integrated Analysis Using Satellite,Aircraft Ozonesonde,and Surface Observations[J].Atmospheric Chemistry and Physics,2008,8:6117-6136.
[39]WANG Y,ZHANG Y,HAO J,et al.Seasonal and Spatial Variability of Surface Ozone over China:Contributions from Background and Domestic Pollution[J].Atmospheric Chemistry and Physics,2011,11:3511-3525.
[40]JIANG Z,MIYAZAKI K,WORDEN J R,et al.Impacts of Anthropogenic and Natural Sources on Free Tropospheric Ozone over the Middle East[J].Atmospheric Chemistry and Physics,2016,16:6537-6546.
[41]ZHANG Q,STREETS D G,CARMICHAEL G R,et al.Asian Emissions in 2006 for the NASA INTEX-B Mission[J].Atmospheric Chemistry and Physics,2009,9:5131-5153.
[42]VAN DER WERF G R,RANDERSON J T,GIGLIO L,et al.Global fire Emissions and the Contribution of Deforestation,Savanna,Forest,Agricultural,and Peat Fires(1997-2009)[J].Atmospheric Chemistry and Physics,2010,10:11707-11735.
[43]GUENTHER A B,JIANG X,HEALD C L,et al.The Model of Emissions of Gases and Aerosols from Nature Version 2.1(MEGAN2.1):An Extended and Updated Framework for Modeling Biogenic Emissions[J].Geoscientific Model Development,2012,5:1471-1492.
[44]ALLEN D,PICKERING K,DUNCAN B,et al.Impact of Lightning NO Emissions on North American Photochemistry as Determined Using the Global Modeling Initiative(GMI)Model[J].Journal of Geophysical Research,2010,115:D22301.
[45]OTT L E,PICKERING K E,STENCHIKOV G L,et al.Production of Lightning NOx and Its Vertical Distribution Calculated from Three-dimensional Cloud-scale Chemical Transport Model Simulations[J].Journal of Geophysical Research,2010,115:288-303.
[46]LI B,GASSER T,CIAIS P,et al.The Contribution of China?s Emissions to Global Climate Forcing[J].Nature531:357-361.
[47]DING A,WANG T.Influence of Stratosphere-to-Troposphere Exchange on the Seasonal Cycle of Surface Ozone at Mount Waliguan in Western China[J].Geophysical Research Letters,2006,33:L03803.
[48]EARL N,SIMMONDS I.Spatial and Temporal Variability and Trends in 2001-2016 Global Fire Activity[J].Journal of Geophysical Research,2018,123:2524-2536.
[49]GIGLIO L,RANDERSON J T,VAN DER WERF G R.Analysis of Daily,Monthly,and Annual Burned Area Using the Fourth-generation Global Fire Emissions Database(GFED4)[J].Journal of Geophysical Research,2013,118:317-328.
[50]蒋美青,陆克定,苏榕,等.我国典型城市群O3污染成因和关键VOCs活性解析[J].科学通报,2018,63(12):1130-1141.
[2]MCLINDEN C A,OLSEN S C,HANNEGAN B,et al.Stratospheric Ozone in 3-D Models:A Simple Chemistry and the Cross-tropopause Flux[J].Journal of Geophysical Research,2000,105:14653-14665.
[3]ZHANG Q,HE K B,HUO H.Cleaning China′s Air[J].Nature,2012,484:161-162.
[4]WANG T,XUE L,BRIMBLECOMBE P,et al.Ozone Pollution in China:A Review of Concentrations,Meteorological Influences,Chemical Precursors,and Effects[J].Science of the Total Environment,2017,575:1582-1596.
[5]CHANG K L,PETROPAVLOVSKIKH I,COOPER O R,et al.Regional Trend Analysis of Surface Ozone Observations from Monitoring Networks in Eastern North America,Europe and East Asia[J].Elementa:Science of the Anthropocene,2017,5:50-72.
[6]GAUDEL A,COOPER O,ANCELLET G,et al.Tropospheric Ozone Assessment Report:Present-day Distribution and Trends of Tropospheric Ozone Relevant to Climate and Global Atmospheric Chemistry Model Evaluation[J].Elementa:Science of the Anthropocene,2018,6:39.
[7]DING A,HUANG X,FU C.Air Pollution and Weather Interaction in East Asia[J].Oxford Research Encyclopedias-Environmental Science,2017,1:1-26.
[8]XU W,XU X,LIN M,et al.Long-term Trends of Surface Ozone and Its Influencing Factors at the Mt Waliguan GAW Station,China-Part 2:The Roles of Anthropogenic Emissions and Climate Variability[J].Atmospheric Chemistry and Physics,2018,18:773-798.
[9]SUN W,SHAO M,GRANIER C,et al.Long-Term Trends of Anthropogenic SO2,NOx,CO,and NMVOCs Emissions in China[J].Earth's Future,2018,6:1112-1133.
[10]ZHENG B,TONG D,LI M,et al.Trends in China's Anthropogenic Emissions Since 2010 as the Consequence of Clean Air Actions[J].Atmospheric Chemistry and Physics,2018,18:14095-14111.
[11]LU X,HONG J,ZHANG L,et al.Severe Surface Ozone Pollution in China:A Global Perspective[J].Environmental Science&Technology Letters,2018,5:487-494.
[12]SEKIYA T,SUDO K.Roles of Transport and Chemistry Processes in Global Ozone Change on Interannual and Multidecadal Time Scales[J].Journal of Geophysical Research,2014,119:4903-4921.
[13]DING A,FU C,YANG X,et al.Ozone and Fine Particle in the Western Yangtze River Delta:An Overview of 1Year Data at the SORPES Station[J].Atmospheric Chemistry and Physics,2013,13:5813-5830.
[14]JIANG Y,ZHAO T,LIU J,et al.Why Does Surface Ozone Peak before a Typhoon Landing in Southeast China[J].Atmospheric Chemistry and Physics,2015,15:13331-13338.
[15]ZHOU D,DING A,MAO H,et al.Impacts of the East Asian Monsoon on Lower Tropospheric Ozone over Coastal South China[J].Environmental Research Letters2013,8:044011.
[16]YANG Y,LIAO H,LI J.Impacts of the East Asian Summer Monsoon on Interannual Variations of Summertime Surface-layer Ozone Concentrations over China[J].Atmospheric Chemistry and Physics,2014,14:6867-6879.
[17]LI S,WANG T,HUANG X,et al.Impact of East Asian Summer Monsoon on Surface Ozone Pattern in China[J].Journal of Geophysical Research,2018,123:1401-1411.
[18]LIU H,JACOB D J,CHAN L Y,et al.Sources of Tropospheric Ozone Along the Asian Pacific Rim:An Analysis of Ozone Sonde Observations[J].Journal of Geophysical Research,2002,107:D21.
[19]FIORE A M,DENTENER F J,WILD O,et al.Multimodel Estimates of Intercontinental Source-receptor Relationships for Ozone Pollution[J].Journal of Geophysical Research,2009,114:D04301.
[20]DOHERTY R M.Ozone Pollution from Near and Far[J].Nature Geoscience,2015,8:664.
[21]HAN H,LIU J,YUAN H,et al.Impacts of Synoptic Weather Patterns and Their Persistency on Free Tropospheric Carbon Monoxide Concentrations and Outflow in Eastern China[J].Journal of Geophysical Research,2018,123:7024-7046.
[22]HAN H,LIU J,YUAN H,et al.Characteristics of Intercontinental Transport of Tropospheric Ozone from Africa to Asia[J].Atmospheric Chemistry and Physics,2018,18:4251-4276.
[23]ZHU Y,LIU J,WANG T,et al.The Impacts of Meteorology on the Seasonal and Interannual Variabilities of Ozone Transport from North America to East Asia[J].Journal of Geophysical Research,2017,122:10612-10636.
[24]YOSHITOMI M,WILD O,AKIMOTO H.Contributions of Regional and Intercontinental Transport to Surface Ozone in the Tokyo Area[J].Atmospheric Chemistry and Physics,2011,11:7583-7599.
[25]NAGASHIMA T,SUDO K,AKIMOTO H,et al.Long-term Change in the Source Contribution to Surface Ozone over Japan[J].Atmospheric Chemistry and Physics,2017,17:8231-8246.
[26]ZHANG L,JACOB D J,KOPACZ M,et al.Intercontinental Source Attribution of Ozone Pollution at Western U.S.Sites Using an Adjoint Method[J].Geophysical Research Letters,2009,36:L11810.
[27]COOPER O R,LANGFORD A O,PARRISH D D,et al.Challenges of a Lowered U.S.Ozone Standard,Science[J].2015,348:1096-1097.
[28]HUANG M,CARMICHAEL G R,PIERCE R B,et al.Impact of Intercontinental Pollution Transport on North American Ozone Air Pollution:An HTAP Phase 2Multi-model Study[J].Atmospheric Chemistry and Physics,2017,17:5721-5750.
[29]DENTENER F,KEATING T,AKIMOTO H.HTAP:Hemispheric Transport of Air Pollution 2010[M].United Nations:New York and Geneva,2010.
[30]NI R,LIN J,YAN Y,et al.Foreign and Domestic Contributions to Springtime Ozone Over China[J].Atmospheric Chemistry and Physics,2018,18:11447-11469.
[31]VAN der WERF G R,RANDERSON J T,GIGLIO L,et al.Global Fire Emissions Estimates during 1997-2016[J].Earth System Science Data,2017,9:697-720.
[32]DING A,FU C,YANG X,et al.Intense Atmospheric Pollution Modifies Weather:A Case of Mixed Biomass Burning with Fossil Fuel Combustion Pollution in Eastern China[J].Atmospheric Chemistry and Physics,2013,13:10545-10554.
[33]HUANG X,DING A,LIU L,et al.Effects of Aerosol-radiation Interaction on Precipitation during Biomass-burning Season in East China[J].Atmospheric Chemistry and Physics,2016,16:10063-10082.
[34]TANG H,LIU G,ZHU J,et al.Seasonal Variations in Surface Ozone as Influenced by Asian Summer Monsoon and Biomass Burning in Agricultural Fields of the Northern Yangtze River Delta[J].Atmospheric Research,2013,122:67-76.
[35]CHAN K.Biomass Burning Sources and Their Contributions to the Local Air Quality in Hong Kong[J].Science of The Total Environment,2017,596-597:212-221.
[36]DING K,LIU J,DING A,et al.Uplifting of Carbon Monoxide from Biomass Burning and Anthropogenic Sources to the Free Troposphere in East Asia[J].Atmospheric Chemistry and Physics,2015,15:2843-2866.
[37]BEY I,JACOB D J,YANTOSCA R M,et al.Global Modeling of Tropospheric Chemistry with Assimilated Meteorology:Model Description and Evaluation[J].Journal of Geophysical Research,2001,106:23073-23095.
[38]ZHANG L,JACOB D J,BOERSMA K F,et al.Transpacific Transport of Ozone Pollution and the Effect of Recent Asian Emission Increases on Air Quality in North America:An Integrated Analysis Using Satellite,Aircraft Ozonesonde,and Surface Observations[J].Atmospheric Chemistry and Physics,2008,8:6117-6136.
[39]WANG Y,ZHANG Y,HAO J,et al.Seasonal and Spatial Variability of Surface Ozone over China:Contributions from Background and Domestic Pollution[J].Atmospheric Chemistry and Physics,2011,11:3511-3525.
[40]JIANG Z,MIYAZAKI K,WORDEN J R,et al.Impacts of Anthropogenic and Natural Sources on Free Tropospheric Ozone over the Middle East[J].Atmospheric Chemistry and Physics,2016,16:6537-6546.
[41]ZHANG Q,STREETS D G,CARMICHAEL G R,et al.Asian Emissions in 2006 for the NASA INTEX-B Mission[J].Atmospheric Chemistry and Physics,2009,9:5131-5153.
[42]VAN DER WERF G R,RANDERSON J T,GIGLIO L,et al.Global fire Emissions and the Contribution of Deforestation,Savanna,Forest,Agricultural,and Peat Fires(1997-2009)[J].Atmospheric Chemistry and Physics,2010,10:11707-11735.
[43]GUENTHER A B,JIANG X,HEALD C L,et al.The Model of Emissions of Gases and Aerosols from Nature Version 2.1(MEGAN2.1):An Extended and Updated Framework for Modeling Biogenic Emissions[J].Geoscientific Model Development,2012,5:1471-1492.
[44]ALLEN D,PICKERING K,DUNCAN B,et al.Impact of Lightning NO Emissions on North American Photochemistry as Determined Using the Global Modeling Initiative(GMI)Model[J].Journal of Geophysical Research,2010,115:D22301.
[45]OTT L E,PICKERING K E,STENCHIKOV G L,et al.Production of Lightning NOx and Its Vertical Distribution Calculated from Three-dimensional Cloud-scale Chemical Transport Model Simulations[J].Journal of Geophysical Research,2010,115:288-303.
[46]LI B,GASSER T,CIAIS P,et al.The Contribution of China?s Emissions to Global Climate Forcing[J].Nature531:357-361.
[47]DING A,WANG T.Influence of Stratosphere-to-Troposphere Exchange on the Seasonal Cycle of Surface Ozone at Mount Waliguan in Western China[J].Geophysical Research Letters,2006,33:L03803.
[48]EARL N,SIMMONDS I.Spatial and Temporal Variability and Trends in 2001-2016 Global Fire Activity[J].Journal of Geophysical Research,2018,123:2524-2536.
[49]GIGLIO L,RANDERSON J T,VAN DER WERF G R.Analysis of Daily,Monthly,and Annual Burned Area Using the Fourth-generation Global Fire Emissions Database(GFED4)[J].Journal of Geophysical Research,2013,118:317-328.
[50]蒋美青,陆克定,苏榕,等.我国典型城市群O3污染成因和关键VOCs活性解析[J].科学通报,2018,63(12):1130-1141.
© 2004-2018 中国地质图书馆版权所有 京ICP备05064691号 京公网安备11010802017129号 地址：北京市海淀区学院路29号 邮编：100083 电话：办公室：(+86 10)66554848；文献借阅、咨询服务、科技查新：66554700 |