长三角地区大气污染物的研究进展
|
摘要
长江三角洲地区(简称长三角地区)作为我国三大经济圈之一,能源消耗的快速增长使大气污染问题日益严重,以颗粒物和O3为主的大气污染问题已成为专家和学者研究的热点问题。从大气污染物的时空分布特征、长距离输送特征以及来源解析3个方面调研了长三角地区大气污染物的研究进展,并就大气污染物研究进展工作提出相关建议及展望。
The Yangtze River Delta( Yangtze River Delta) is one of the three major economic circles in China. The rapid growth of energy consumption has made the problem of air pollution more and more serious.The problem of air pollution,mainly particulates and O3,has become a hot issue for experts and scholars. This paper investigates the research progress of atmospheric pollutants in the Yangtze River Delta from three aspects: the spatial and temporal distribution characteristics of atmospheric pollutants,long-distance transport characteristics and source analysis,and puts forward relevant suggestions and prospects for the research progress of atmospheric pollutants.
The Yangtze River Delta( Yangtze River Delta) is one of the three major economic circles in China. The rapid growth of energy consumption has made the problem of air pollution more and more serious.The problem of air pollution,mainly particulates and O3,has become a hot issue for experts and scholars. This paper investigates the research progress of atmospheric pollutants in the Yangtze River Delta from three aspects: the spatial and temporal distribution characteristics of atmospheric pollutants,long-distance transport characteristics and source analysis,and puts forward relevant suggestions and prospects for the research progress of atmospheric pollutants.
引文
[1]WANG T,CHEUNG V T F,ANSON M,et al.Ozone and related gaseous pollutants in the boundary layer of Eastern China:overview of the recent measurements at a rural site[J].Geophysical Research Letters,2001,28(12):2373-2376.
[2]TIE X,BRASSEUR G,ZHAO C,et al.Chemical characterization of air pollution in Eastern China and the Eastern United States[J]. Atmospheric Environment,2006,40(14):2607-2625.
[3]CHAN C K,YAO X.Air pollution in mega cities in China[J].Atmospheric Environment,2008,42(1):1-41.
[4]XIAO Z M,ZHANG Y F,HONG S M,et al.Estimation of the main factors influencing haze,based on a long-term monitoring campaign in Hangzhou,China[J]. Aerosol&Air Quality Research,2011,11(7):873-882.
[5]ZHAO W,CHENG J,GUO M,et al.Ambient air particulate matter in the yangtze river delta region,China:spatial,annual,and seasonal variations and health risks[J].Environmental Engineering Science,2011,28(11):795-802.
[6]HUANG K,ZHUANG G,LIN Y,et al.Typical types and formation mechanisms of haze in an Eastern Asia megacity,Shanghai[J]. Atmospheric Chemistry&Physics Discussions,2011,11(8):21713-21767.
[7]杨俊梅,李培仁,李义宇,等.南京北郊O3、NO2和SO2变化特征分析[J].气象环境学报,2014,30(3):66-70.
[8]DING A J,FU C B,YANG X Q,et al.Ozone and fine particle in the western Yangtze River Delta:an overview of 1-yr data at the SORPES station[J].Atmospheric Chemistry&Physics,2013,13(11):5813-5830.
[9]易睿,王亚林,张殷俊,等.长江三角洲地区城市臭氧污染特征与影响因素分析[J].环境科学学报,2015,35(8):2370-2377.
[10]张纬,郭胜利,申付振,等.南京地区PM2. 5和PM10浓度分布特征及与相关气象条件的关系[J].科学技术与工程,2016,16(4):124-129.
[11]胡森林,刘红年.合肥市PM2. 5对城市辐射和气温的影响[J].气象科学,2017,37(1):78-85.
[12]花艳,潘良宝,汤莉莉,等.南京霾天颗粒物数浓度特征及其受气象条件影响分析[J].气象科学,2017,37(3):385-393.
[13]王自发,庞成明,朱江,等.大气环境数值模拟研究新进展[J].大气科学,2008,32(4):987-995.
[14]程真,陈长虹,黄成,等.长三角区域城市间一次污染跨界影响[J].环境科学学报.2011,31(4):686-694.
[15]GRELL G A,PECKHAM S E,SCHMITZ R,et al. Fully coupled“online”chemistry within the WRF mode[J]. Atmospheric Environment,2005,39(37):6957-6975.
[16]TIE X X,GENG F H,LI P,et al.Measurement and modeling of O3variability in Shanghai,China:application of the WRF-chem model[J].Atmospheric Environment,2009,43(28):4289-4302.
[17]张亮,朱彬,高晋徽,等.长江三角洲夏季一次典型臭氧污染过程的模拟[J].环境科学,2015,36(11):3981-3988.
[18]李锋,朱彬,安俊岭,等.2013年12月初长江三角洲及周边地区重霾污染的数值模拟[J].中国环境科学,2015,35(7):1965-1974.
[19]王占山,李晓倩,王宗爽,等.空气质量模型CMAQ的国内外研究现状[J].环境科学与技术,2013,36(6L):386-391.
[20]李莉,陈长虹,黄成,等.长江三角洲地区大气O3和PM10的区域污染特征模拟[J].环境科学.2008,29(1):237-245.
[21]HUANG C,CHEN C H,LI L,et al.Emission inventory of anthropogenic air pollutants and VOC species in the Yangtze River Delta region,China[J]. Atmospheric Chemistry and Physics.2011,11(9):4105-4120.
[22]李莉,陈长虹,黄海英.应用Models-3/CMAQ研究长三角区域大气污染及输送[J].上海环境科学,2007(4):159-165.
[23]张艳,余琦,伏晴艳,等.长江三角洲区域输送对上海市空气质量影响的特征分析[J].中国环境科学,2010,30(7):914-923.
[24]王自发,谢付莹,王喜全,等.嵌套网格空气质量预报模式系统的发展与应用[J].大气科学,2006,30(5):778-790.
[25]李杰,杨文夷,陈焕盛,等.东亚大气可吸入颗粒物时空分布的数值模拟研究[J].环境科学学报,2014,34(3):548-557.
[26]杨文夷,李杰,陈焕盛,等.东亚边界层臭氧时空分布的数值模拟研究[J].中国环境科学,2014,34(7):1633-1641.
[27]边智,李杰,王喜全,等.泰山春季臭氧污染特征[J].环境科学研究,2006(5):36-39.
[28]MOODY J L,GALLOWAY J N. Quantifying the relationship between atmospheric transport and the chemical composition of precipitation on Bermuda[J]. Tellus Series Bchemical&Physical Meteorology,1958,40b(5):463-479.
[29]王艳,柴发合,刘厚凤,等.长江三角洲地区大气污染物水平输送场特征分析[J].环境科学研究.2008,21(1):22-29.
[30]刘世玺,安俊琳,朱彬,等.远距离输送作用对南京大气污染的影响[J].生态环境学报,2011,19(11):2629-2635.
[31]王茜.利用轨迹模式研究上海大气污染的输送来源[J].环境科学研究,2013(4):357-363.
[32]方利江,傅贤康,谢立峰,等.舟山本岛大气污染输送过程的数值模拟分析[J].环境科学研究,2014,27(10):1087-1094.
[33]安静宇,李莉,黄成,等.2013年1月中国东部地区重污染过程中上海市细颗粒物的来源追踪模拟研究[J].环境科学学报,2014,34(10):2635-2644.
[34]樊曙先,徐建强,郑有飞,等.南京市气溶胶PM2. 5一次来源解析[J].气象科学,2005,25(6):588-593.
[35]张光亮,耿存珍.大气颗粒物源解析CMB法与PFA法原理及比较研究[J].环境巧学与管理,2014,39(10):56-59.
[36]唐邀.天津市环境空气PM2. 5来源解析[D].天津:南开大学,2014.
[37]张延君,郑玫,蔡靖,等.PM2. 5源解祈方法的比較与评述机[J].科学通报,2015,60(2):109-121.
[38]WANG Y,LI L,CHEN C,et al. Source apportionment of fine particulate matter during autumn haze episodes in Shanghai,China:source apportionment[J].Journal of Geophysical Research Atmospheres,2014,119(4):1903-1914.
[39]MILLER M S,FRIEDLANDER S K,HIDY G M.A chemical element balance for the Pasadena aerosol[J]. Journal of Colloid and Interface Science,1972,39:165-176.
[40]PAATERO P,TAPPER U. Analysis of different modes of factor analysis as least square fit problems[J].Chemometrics Intelligent Laboratory Systems,1993,18(2):183-194.
[41]肖致美,毕晓辉,冯银厂,等.宁波市环境空气中PM10和PM2. 5来源解析[J].环境科学研究,2012,25(5):549-555.
[42]王苏蓉,喻义勇,王勤耕,等.基于PMF模式的南京市大气细颗粒物源解析[J].中国环境科学,2015,35(12):3535-3542.
[43]LI J,WANG Z F,AKIMOTO H,et al.Near-ground ozone source attributions and outflow in central eastern China during MTX2006[J].Atmospheric Chemistry and Physics,2008,8(24):7335-7351.
[2]TIE X,BRASSEUR G,ZHAO C,et al.Chemical characterization of air pollution in Eastern China and the Eastern United States[J]. Atmospheric Environment,2006,40(14):2607-2625.
[3]CHAN C K,YAO X.Air pollution in mega cities in China[J].Atmospheric Environment,2008,42(1):1-41.
[4]XIAO Z M,ZHANG Y F,HONG S M,et al.Estimation of the main factors influencing haze,based on a long-term monitoring campaign in Hangzhou,China[J]. Aerosol&Air Quality Research,2011,11(7):873-882.
[5]ZHAO W,CHENG J,GUO M,et al.Ambient air particulate matter in the yangtze river delta region,China:spatial,annual,and seasonal variations and health risks[J].Environmental Engineering Science,2011,28(11):795-802.
[6]HUANG K,ZHUANG G,LIN Y,et al.Typical types and formation mechanisms of haze in an Eastern Asia megacity,Shanghai[J]. Atmospheric Chemistry&Physics Discussions,2011,11(8):21713-21767.
[7]杨俊梅,李培仁,李义宇,等.南京北郊O3、NO2和SO2变化特征分析[J].气象环境学报,2014,30(3):66-70.
[8]DING A J,FU C B,YANG X Q,et al.Ozone and fine particle in the western Yangtze River Delta:an overview of 1-yr data at the SORPES station[J].Atmospheric Chemistry&Physics,2013,13(11):5813-5830.
[9]易睿,王亚林,张殷俊,等.长江三角洲地区城市臭氧污染特征与影响因素分析[J].环境科学学报,2015,35(8):2370-2377.
[10]张纬,郭胜利,申付振,等.南京地区PM2. 5和PM10浓度分布特征及与相关气象条件的关系[J].科学技术与工程,2016,16(4):124-129.
[11]胡森林,刘红年.合肥市PM2. 5对城市辐射和气温的影响[J].气象科学,2017,37(1):78-85.
[12]花艳,潘良宝,汤莉莉,等.南京霾天颗粒物数浓度特征及其受气象条件影响分析[J].气象科学,2017,37(3):385-393.
[13]王自发,庞成明,朱江,等.大气环境数值模拟研究新进展[J].大气科学,2008,32(4):987-995.
[14]程真,陈长虹,黄成,等.长三角区域城市间一次污染跨界影响[J].环境科学学报.2011,31(4):686-694.
[15]GRELL G A,PECKHAM S E,SCHMITZ R,et al. Fully coupled“online”chemistry within the WRF mode[J]. Atmospheric Environment,2005,39(37):6957-6975.
[16]TIE X X,GENG F H,LI P,et al.Measurement and modeling of O3variability in Shanghai,China:application of the WRF-chem model[J].Atmospheric Environment,2009,43(28):4289-4302.
[17]张亮,朱彬,高晋徽,等.长江三角洲夏季一次典型臭氧污染过程的模拟[J].环境科学,2015,36(11):3981-3988.
[18]李锋,朱彬,安俊岭,等.2013年12月初长江三角洲及周边地区重霾污染的数值模拟[J].中国环境科学,2015,35(7):1965-1974.
[19]王占山,李晓倩,王宗爽,等.空气质量模型CMAQ的国内外研究现状[J].环境科学与技术,2013,36(6L):386-391.
[20]李莉,陈长虹,黄成,等.长江三角洲地区大气O3和PM10的区域污染特征模拟[J].环境科学.2008,29(1):237-245.
[21]HUANG C,CHEN C H,LI L,et al.Emission inventory of anthropogenic air pollutants and VOC species in the Yangtze River Delta region,China[J]. Atmospheric Chemistry and Physics.2011,11(9):4105-4120.
[22]李莉,陈长虹,黄海英.应用Models-3/CMAQ研究长三角区域大气污染及输送[J].上海环境科学,2007(4):159-165.
[23]张艳,余琦,伏晴艳,等.长江三角洲区域输送对上海市空气质量影响的特征分析[J].中国环境科学,2010,30(7):914-923.
[24]王自发,谢付莹,王喜全,等.嵌套网格空气质量预报模式系统的发展与应用[J].大气科学,2006,30(5):778-790.
[25]李杰,杨文夷,陈焕盛,等.东亚大气可吸入颗粒物时空分布的数值模拟研究[J].环境科学学报,2014,34(3):548-557.
[26]杨文夷,李杰,陈焕盛,等.东亚边界层臭氧时空分布的数值模拟研究[J].中国环境科学,2014,34(7):1633-1641.
[27]边智,李杰,王喜全,等.泰山春季臭氧污染特征[J].环境科学研究,2006(5):36-39.
[28]MOODY J L,GALLOWAY J N. Quantifying the relationship between atmospheric transport and the chemical composition of precipitation on Bermuda[J]. Tellus Series Bchemical&Physical Meteorology,1958,40b(5):463-479.
[29]王艳,柴发合,刘厚凤,等.长江三角洲地区大气污染物水平输送场特征分析[J].环境科学研究.2008,21(1):22-29.
[30]刘世玺,安俊琳,朱彬,等.远距离输送作用对南京大气污染的影响[J].生态环境学报,2011,19(11):2629-2635.
[31]王茜.利用轨迹模式研究上海大气污染的输送来源[J].环境科学研究,2013(4):357-363.
[32]方利江,傅贤康,谢立峰,等.舟山本岛大气污染输送过程的数值模拟分析[J].环境科学研究,2014,27(10):1087-1094.
[33]安静宇,李莉,黄成,等.2013年1月中国东部地区重污染过程中上海市细颗粒物的来源追踪模拟研究[J].环境科学学报,2014,34(10):2635-2644.
[34]樊曙先,徐建强,郑有飞,等.南京市气溶胶PM2. 5一次来源解析[J].气象科学,2005,25(6):588-593.
[35]张光亮,耿存珍.大气颗粒物源解析CMB法与PFA法原理及比较研究[J].环境巧学与管理,2014,39(10):56-59.
[36]唐邀.天津市环境空气PM2. 5来源解析[D].天津:南开大学,2014.
[37]张延君,郑玫,蔡靖,等.PM2. 5源解祈方法的比較与评述机[J].科学通报,2015,60(2):109-121.
[38]WANG Y,LI L,CHEN C,et al. Source apportionment of fine particulate matter during autumn haze episodes in Shanghai,China:source apportionment[J].Journal of Geophysical Research Atmospheres,2014,119(4):1903-1914.
[39]MILLER M S,FRIEDLANDER S K,HIDY G M.A chemical element balance for the Pasadena aerosol[J]. Journal of Colloid and Interface Science,1972,39:165-176.
[40]PAATERO P,TAPPER U. Analysis of different modes of factor analysis as least square fit problems[J].Chemometrics Intelligent Laboratory Systems,1993,18(2):183-194.
[41]肖致美,毕晓辉,冯银厂,等.宁波市环境空气中PM10和PM2. 5来源解析[J].环境科学研究,2012,25(5):549-555.
[42]王苏蓉,喻义勇,王勤耕,等.基于PMF模式的南京市大气细颗粒物源解析[J].中国环境科学,2015,35(12):3535-3542.
[43]LI J,WANG Z F,AKIMOTO H,et al.Near-ground ozone source attributions and outflow in central eastern China during MTX2006[J].Atmospheric Chemistry and Physics,2008,8(24):7335-7351.