核废料储罐表面化学环境长期演变预测
|
摘要
通过对国内外的核废料处置库环境试验监测及预测模型的调研,总结了核废料储罐在直接填埋、缓冲/回填和加混凝土缓冲层等埋藏方式下的表面环境变化,主要包括氧含量、缓冲材料的孔隙液成分及pH值,为我国核废料储库环境下储罐表面重要的腐蚀演变研究提供了参考。
Surface environment changes of nuclear waste container, mainly including oxygen contents, buffer pore water components and pH under the conditions of "borehole" type and "In-floor" type with bentonite buffer/backfill and concrete buffer were summarized. This summarization provides a basic corrosion environment reference for the corrosion evolution research of high-level radioactive waste disposal repository in our country.
Surface environment changes of nuclear waste container, mainly including oxygen contents, buffer pore water components and pH under the conditions of "borehole" type and "In-floor" type with bentonite buffer/backfill and concrete buffer were summarized. This summarization provides a basic corrosion environment reference for the corrosion evolution research of high-level radioactive waste disposal repository in our country.
引文
[1]史永谦.核能发电的优点及世界核电发展动向[J].能源工程,2007(1):1-6.
[2]COHEN B L,施向军.核电的优越性[J].中国核工业,2000(3):54-55.
[3]DUQUETTE D J,LATANISION R M,DI BELLA C AW,et al.Corrosion Issues Related to Disposal of High-level Nuclear Waste in the Yucca Mountain Repository-Peer Reviewer’s Perspective[J].Corrosion,2009,65(4):272-280.
[4]SKB.Sea Disposal of Radioactive Wastes(Technical Report TR-01-30)[R].Vienna:IAEA Bulletin 2/1994,2001.
[5]LAURENT De W,FRAN?OIS M,JéR?ME C,et al.Modeling of Oxygen Gas Diffusion and Consumption during the Oxic Transient in a Disposal Cell of Radioactive Waste[J].Applied Geochemistry,2014,41:115-127.
[6]YANG C B,JAVIER S,JORGE M,et al.Modeling Geochemical and Microbial Consumption of Dissolved Oxygen after Backfilling a High Level Radioactive Waste Repository[J].Journal of Contaminant Hydrology,2007,93:130-148.
[7]ROSBORG B,WERME L.The Swedish Nuclear Waste Program and the Long-term Corrosion Behaviour of Copper[J].Journal of Nuclear Materials,2008,379:142-153.
[8]郭永海,王驹,肖丰,等.高放废物处置库甘肃北山预选区地下水的形成[J].高校地质学报,2010,16(1):13-18.
[9]郭永海,王驹,王志明,等.高放废物处置库甘肃北山预选区地下水位动态特征[J].铀矿地质,2010,26(1):46-59.
[10]董艳辉,李国敏,黎明.甘肃北山大区域地下水流动模拟[J].科学通报,2009,54(23):3790-3792.
[11]赵春虎,李国敏,郭永海,等.甘肃北山区域地下水流动特征[J].工程地质学报,2007,15(2):174-178.
[12]庞忠和,郭永海,苏锐,等.北山花岗岩裂隙地下水循环属性试验研究[J].岩石力学与工程学报,2007,26(2):3954-3958.
[13]王海龙.高放废物处置库北山预选区区域地下水流模拟及岩体渗透特征研究[D].北京:核工业北京地质研究院,2014.
[14]郑珉,张琦超,黄彦良,等.中国高放废物处置库甘肃北山预选区腐蚀研究用代表性地下水成分的确定[J].中国腐蚀与防护学报,2016,36(2):185-190.
[15]SEETHARAM S C,CLEALL P J,THOMAS H R.Modelling Some Aspects of Ion Migration in a Compacted Bentonitic Clay[J].Engineering Geology,2006,85:221-228.
[16]KURSTEN B,DRUYTS F.Methodology to Make a Robust Estimation of the Carbon Steel Overpack Life Time with Respect to the Belgian Super Container Design[J].Journal of Nuclear Materials,2008,379:91-96.
[17]TROTIGNON L,DEVALLOIS V,PEYCELON H,et al.Predicting the Long Term Durability of Concrete Engineered Barriers in a Geological Repository for Radioactive Waste[J].Physics and Chemistry of the Earth,2007,32:259-274.
[18]BERNER U,DMITRII A K,GEORG K.Geochemical Impact of a Low-pH Cement Liner on the Near Field of a Repository for Spent Fuel and High-level Radioactive Waste[J].Physics and Chemistry of the Earth,2013,64:46-56.
[19]BERNER U.Setting up Bentonite Pore Water Compositions(Internal report AN-44-10-04)[R].Villigen:Paul Scherrer Institute,2010.
[20]YANG C,SAMPER J,MONTENEGRO L.A Coupled Non-isothermal Reactive Transport Model for Long-term Geochemical Evolution of a HLW Repository in Clay[J].Environmental Geology,2008,53(8):1627-1638.
[2]COHEN B L,施向军.核电的优越性[J].中国核工业,2000(3):54-55.
[3]DUQUETTE D J,LATANISION R M,DI BELLA C AW,et al.Corrosion Issues Related to Disposal of High-level Nuclear Waste in the Yucca Mountain Repository-Peer Reviewer’s Perspective[J].Corrosion,2009,65(4):272-280.
[4]SKB.Sea Disposal of Radioactive Wastes(Technical Report TR-01-30)[R].Vienna:IAEA Bulletin 2/1994,2001.
[5]LAURENT De W,FRAN?OIS M,JéR?ME C,et al.Modeling of Oxygen Gas Diffusion and Consumption during the Oxic Transient in a Disposal Cell of Radioactive Waste[J].Applied Geochemistry,2014,41:115-127.
[6]YANG C B,JAVIER S,JORGE M,et al.Modeling Geochemical and Microbial Consumption of Dissolved Oxygen after Backfilling a High Level Radioactive Waste Repository[J].Journal of Contaminant Hydrology,2007,93:130-148.
[7]ROSBORG B,WERME L.The Swedish Nuclear Waste Program and the Long-term Corrosion Behaviour of Copper[J].Journal of Nuclear Materials,2008,379:142-153.
[8]郭永海,王驹,肖丰,等.高放废物处置库甘肃北山预选区地下水的形成[J].高校地质学报,2010,16(1):13-18.
[9]郭永海,王驹,王志明,等.高放废物处置库甘肃北山预选区地下水位动态特征[J].铀矿地质,2010,26(1):46-59.
[10]董艳辉,李国敏,黎明.甘肃北山大区域地下水流动模拟[J].科学通报,2009,54(23):3790-3792.
[11]赵春虎,李国敏,郭永海,等.甘肃北山区域地下水流动特征[J].工程地质学报,2007,15(2):174-178.
[12]庞忠和,郭永海,苏锐,等.北山花岗岩裂隙地下水循环属性试验研究[J].岩石力学与工程学报,2007,26(2):3954-3958.
[13]王海龙.高放废物处置库北山预选区区域地下水流模拟及岩体渗透特征研究[D].北京:核工业北京地质研究院,2014.
[14]郑珉,张琦超,黄彦良,等.中国高放废物处置库甘肃北山预选区腐蚀研究用代表性地下水成分的确定[J].中国腐蚀与防护学报,2016,36(2):185-190.
[15]SEETHARAM S C,CLEALL P J,THOMAS H R.Modelling Some Aspects of Ion Migration in a Compacted Bentonitic Clay[J].Engineering Geology,2006,85:221-228.
[16]KURSTEN B,DRUYTS F.Methodology to Make a Robust Estimation of the Carbon Steel Overpack Life Time with Respect to the Belgian Super Container Design[J].Journal of Nuclear Materials,2008,379:91-96.
[17]TROTIGNON L,DEVALLOIS V,PEYCELON H,et al.Predicting the Long Term Durability of Concrete Engineered Barriers in a Geological Repository for Radioactive Waste[J].Physics and Chemistry of the Earth,2007,32:259-274.
[18]BERNER U,DMITRII A K,GEORG K.Geochemical Impact of a Low-pH Cement Liner on the Near Field of a Repository for Spent Fuel and High-level Radioactive Waste[J].Physics and Chemistry of the Earth,2013,64:46-56.
[19]BERNER U.Setting up Bentonite Pore Water Compositions(Internal report AN-44-10-04)[R].Villigen:Paul Scherrer Institute,2010.
[20]YANG C,SAMPER J,MONTENEGRO L.A Coupled Non-isothermal Reactive Transport Model for Long-term Geochemical Evolution of a HLW Repository in Clay[J].Environmental Geology,2008,53(8):1627-1638.