地下水除铁除锰方法的研究进展
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摘要
介绍了吸附法中吸附剂的处理原理与效果(锰砂、沸石、火山岩、生物质和活性炭等),分析了生物法中的微生物及影响因素,回顾了氧化法中的三大氧化处理方法(自然氧化法、接触氧化法、药剂氧化法),简述了膜技术法和其他新方法。文章结论中,分别指出了吸附法、生物法、氧化法和膜技术法今后的研究方向。吸附法今后的研究重心可继续放在改性上;生物法今后的研究方向可以以培养出超级菌为目标,以应对复杂的地下水水质;氧化法可以将重心放在氧化药剂和其他技术联合处理上;膜技术法今后研究重点是膜污染,可从膜污染的清洗和预防膜污染方面着手。
In this article, we introduce the adsorption of adsorbent processing principle and effect(manganese sand, zeolite, volcanic rock, biomass and activated carbon, etc.), analyze the microbial and influence factors of biological method, reviews the three oxidation oxidation treatment method(natural oxidation, contact oxidation, chemical oxidation method), describes the membrane technology and other new methods. At the end of this article, the research directions of adsorption method, biological method, oxidation method and membrane technology are suggested.
In this article, we introduce the adsorption of adsorbent processing principle and effect(manganese sand, zeolite, volcanic rock, biomass and activated carbon, etc.), analyze the microbial and influence factors of biological method, reviews the three oxidation oxidation treatment method(natural oxidation, contact oxidation, chemical oxidation method), describes the membrane technology and other new methods. At the end of this article, the research directions of adsorption method, biological method, oxidation method and membrane technology are suggested.
引文
[1]Liu J,Zhang H L,You K,et al.Different filter material on the northeast biological iron manganese removal effect of groundwater in the countryside[J].Applied Mechanics and Materials,2014,522:465-468.
[2]赵海华,刘林斌.生物法去除地下水铁锰的影响因素研究[J].工程建设与设计,2013(3):128-130.
[3]赵玉华,常启雷,林长宇,等.Na Cl改性沸石对含铁锰微污染地下水处理效能[J].沈阳建筑大学学报:自然科学版,2010,26(5):966-970.
[4]赵玉华,常启雷,李妍,等.Na OH改性沸石吸附地下水中铁锰效能研究[J].辽宁化工,2009,38(12):857-860.
[5]许景寒,瞿东惠,杨文平.微波加热酸、碱、盐改性沸石对亚铁离子的吸附研究[J].化学与生物工程,2013,30(9):65-67.
[6]胡建龙,王春荣,何绪文,等.改性火山岩滤料去除矿井水中铁锰离子影响因素研究[J].环境工程学报,2009,3(7):1199-1202.
[7]胡建龙,王春荣,何绪文,等.涂铁改性火山岩去除矿井水中铁锰离子试验[J].煤炭科学技术,2009,37(4):114-116.
[8]Abdul Kadir A,Othman N,M Azmi N A.Potential of Using ROSA centifolia to remove iron and manganese in Groundwater Treatment[J].International Journal of Sustainable Construction Engineering and Technology,2012,3(2):70-82.
[9]韩永和,章文贤,周志华,等.凤眼莲对二价铁锰离子的吸附及机理研究[J].环境科学学报,2013,33(3):715-724.
[10]赵良元,朱迟,蒋金辉,等.Bio-F生物吸附剂对水中铁锰的去除与特性[J].环境科学研究,2012,25(4):425-430.
[11]Das B,Hazarika P,Saikia G,et al.Removal of iron from groundwater by ash:A systematic study of a traditional method[J].Journal of Hazardous Materials,2007,141(3):834-841.
[12]bin Jusoh A,Cheng W H,Low W M,et al.Study on the removal of iron and manganese in groundwater by granular activated carbon[J].Desalination,2005,182(1):347-353.
[13]徐越群,赵宏杰,徐菲,等.高锰地下水吸附试验研究[J].南水北调与水利科技,2013(3):35-38.
[14]张吉库,宋鑫,姜阳,等.硅碳素对地下水中Mn2+的吸附研究[J].给水排水,2010,36(增刊):18-21.
[15]霍威.硅碳素滤料在处理地下水中的应用研究[J].节能,2012,31(5):32-34.
[16]Wang Y,Sikora S,Kim H,et al.Effects of solution chemistry on the removal reaction between calcium carbonate-based materials and Fe(II)[J].Science of the Total Environment,2013,443:717-724.
[17]Valentukeviciene M.Experimental research on removal of iron and ammonium ions from groundwater by natural silica sand[J].Geologija,2008,50(3).
[18]赖坤容,李梦耀,周维博.壳聚糖对高锰地下水的吸附研究[J].应用化工,2010,39(8):1167-1169.
[19]Li X,Chu Z,Liu Y,et al.Molecular characterization of microbial populations in full-scale biofilters treating iron,manganese and ammonia containing groundwater in Harbin,China[J].Bioresource Technology,2013,147:234-239.
[20]杨柳,储昭瑞,任玉辉,等.生物滤池同步去除地下水中Fe2+、Mn2+和As(Ⅲ)的试验研究[J].给水排水,2014,40(3):121-124.
[21]Fu J X,Shang J,Zhao Y H.Simultaneous removal of iron,manganese and ammonia from groundwater in single biofilter layer using BAF[J].Advanced Materials Research,2011,183:442-446.
[22]张建林,李相昆,曾辉平,等.高铁高锰微污染地下水的生物同层净化研究[J].中国给水排水,2011,27(21):5-7.
[23]付伟,李金成,叶雪松,等.生物除锰滤层快速启动中营养投加的效果分析[J].青岛理工大学学报,2013,34(5):76-81.
[24]李灿波,王德生,高进仑,等.生物滤池地下水除铁除锰过程中漏锰现象研究[J].供水技术,2012,6(1):16-19.
[25]商俊,傅金祥,赵玉华,等.BAF工艺处理微污染含铁锰地下水试验研究[J].供水技术,2011,5(2):8-11.
[26]Phatai P,Wittayakun J,Chen W H,et al.Removal of manganese(II)and iron(II)from synthetic groundwater using potassium permanganate[J].Desalination and Water Treatment,2014,52(31-33):5942-5951.
[27]赵焱,李冬,李相昆,等.高效生物除铁除锰工程菌MSB-4的特性研究[J].中国给水排水,2009,25(1):40-44.
[28]Hiiob M,Karro E.Iron in the Middle Devonian aquifer system and its removal at voru county water treatment plants,Estonia[J].Estonian Journal of Earth Sciences,2012,61(3):181.
[29]Burke V,Duennbier U,Massmann G.The effect of aeration on the removal of wastewater-derived pharmaceutical residues from groundwater-a laboratory study[J].Water Science&Technology,2012,67(3):658-666.
[30]Dung N T K,Con T H,Cam B D,et al.Investigation of As,Mn and Fe fixation inside the aquifer during groundwater exploitation in the experimental system imitated natural conditions[J].Environmental Geochemistry and Health,2012,34(3):349-354.
[31]李继震.接触氧化除铁除锰机理的探讨[J].中国给水排水,2010,26(18):6-8.
[32]陈旭.接触氧化法除铁的滤料选择[J].中国新技术新产品,2009,(17):64-64.
[33]熊斌,李星,杨艳玲,等.接触氧化/超滤除铁除锰组合工艺的净化效能[J].中国给水排水,2014,30(1):30-33.
[34]汪洋,黄廷林,文刚.地下水中氨氮、铁、锰的同步去除及其相互作用[J].中国给水排水,2014,30(19):32-39.
[35]王娟珍,薛长安,王志勇,等.高锰酸钾应用于地下水除铁锰试验研究与探讨[J].城镇供水,2013(3):78-80.
[36]Ellis D,Bouchard C,Lantagne G.Removal of iron and manganese from groundwater by oxidation and microfiltration[J].Desalination,2000,130(3):255-264.
[37]沈志余,江锐,王颖,等.高锰酸钾除锰方法在水厂生产中的运用[J].供水技术,2014,8(4):18-21.
[38]吴彦志,李雨时.Fenton试剂-石英砂工艺处理高浓度铁锰地下水[J].科技创新导报,2012(9):132-132.
[39]张俊洁,肖利萍.Fenton试剂和锰砂协同处理铁锰矿井废水的研究[J].水资源与水工程学报,2010,21(5):87-89.
[40]赵玉华,陈芳,李艳凤,等.化学氧化法处理高铁锰微污染地下水的实验[J].沈阳建筑大学学报:自然科学版,2012,28(6):1098-1102.
[41]郦丹,余健,张浩江.氯接触氧化过滤去除原水中锰的试验研究[J].工业水处理,2013,33(10):23-26.
[42]崔恒,郑西来,陈蕾,等.二氧化氯-接触催化氧化联合去除水中铁和锰[J].环境工程学报,2014,8(6):2478-2484.
[43]唐玉兰,武利,傅金祥,等.二氧化氯/混凝剂工艺处理含铁水的试验研究[J].供水技术,2010,4(1):14-16.
[44]薛长安,王娟珍,王志勇.次氯酸钠应用于地下水除铁锰试验研究[J].海峡科技与产业,2013(7):60-61.
[45]Kuberis E A,Gorbachov E A.Environmental monitoring and analysis of quality of the Nizhny Novgorod region ground water with the development of the technologies of their filtration[J].Journal of the Geographical Institute Jovan Cvijic,SASA,2014,64(2):177-191.
[46]Lin J L,Huang C,Pan J R,et al.Fouling mitigation of a dead-end microfiltration by mixing-enhanced preoxidation for Fe and Mn removal from groundwater[J].Colloids and Surfaces A:Physicochemical and Engineering Aspects,2013,419:87-93.
[47]李荧,程家迪,刘锐,等.微滤膜处理铁污染地下水的效果及膜污染控制研究[J].中国给水排水,2010,26(1):36-39.
[48]郭绍东,梁恒,陈杰,等.超滤膜组合工艺处理含铁地下水的效能[J].中国给水排水,2014,30(17):5-8.
[49]Rott U,Meyer C,Friedle M.Residue-free removal of arsenic,iron,manganese and ammonia from groundwater[J].Water Supply,2002,2(1):17-24.
[50]狄军贞,马龙,李爱华,等.铁屑+粉煤灰处理含高浓度铁锰氨氮废水试验研究[J].非金属矿,2012,35(4):61-63.
[51]Munter R,Ojaste H,Sutt J.Complexed iron removal from groundwater[J].Journal of Environmental Engineering,2005,131(7):1014-1020.
[52]Piispanen J K,Sallanko J T.Mn(II)removal from groundwater with manganese oxide-coated filter media[J].Journal of Environmental Science and Health Part A,2010,45(13):1732-1740.
[2]赵海华,刘林斌.生物法去除地下水铁锰的影响因素研究[J].工程建设与设计,2013(3):128-130.
[3]赵玉华,常启雷,林长宇,等.Na Cl改性沸石对含铁锰微污染地下水处理效能[J].沈阳建筑大学学报:自然科学版,2010,26(5):966-970.
[4]赵玉华,常启雷,李妍,等.Na OH改性沸石吸附地下水中铁锰效能研究[J].辽宁化工,2009,38(12):857-860.
[5]许景寒,瞿东惠,杨文平.微波加热酸、碱、盐改性沸石对亚铁离子的吸附研究[J].化学与生物工程,2013,30(9):65-67.
[6]胡建龙,王春荣,何绪文,等.改性火山岩滤料去除矿井水中铁锰离子影响因素研究[J].环境工程学报,2009,3(7):1199-1202.
[7]胡建龙,王春荣,何绪文,等.涂铁改性火山岩去除矿井水中铁锰离子试验[J].煤炭科学技术,2009,37(4):114-116.
[8]Abdul Kadir A,Othman N,M Azmi N A.Potential of Using ROSA centifolia to remove iron and manganese in Groundwater Treatment[J].International Journal of Sustainable Construction Engineering and Technology,2012,3(2):70-82.
[9]韩永和,章文贤,周志华,等.凤眼莲对二价铁锰离子的吸附及机理研究[J].环境科学学报,2013,33(3):715-724.
[10]赵良元,朱迟,蒋金辉,等.Bio-F生物吸附剂对水中铁锰的去除与特性[J].环境科学研究,2012,25(4):425-430.
[11]Das B,Hazarika P,Saikia G,et al.Removal of iron from groundwater by ash:A systematic study of a traditional method[J].Journal of Hazardous Materials,2007,141(3):834-841.
[12]bin Jusoh A,Cheng W H,Low W M,et al.Study on the removal of iron and manganese in groundwater by granular activated carbon[J].Desalination,2005,182(1):347-353.
[13]徐越群,赵宏杰,徐菲,等.高锰地下水吸附试验研究[J].南水北调与水利科技,2013(3):35-38.
[14]张吉库,宋鑫,姜阳,等.硅碳素对地下水中Mn2+的吸附研究[J].给水排水,2010,36(增刊):18-21.
[15]霍威.硅碳素滤料在处理地下水中的应用研究[J].节能,2012,31(5):32-34.
[16]Wang Y,Sikora S,Kim H,et al.Effects of solution chemistry on the removal reaction between calcium carbonate-based materials and Fe(II)[J].Science of the Total Environment,2013,443:717-724.
[17]Valentukeviciene M.Experimental research on removal of iron and ammonium ions from groundwater by natural silica sand[J].Geologija,2008,50(3).
[18]赖坤容,李梦耀,周维博.壳聚糖对高锰地下水的吸附研究[J].应用化工,2010,39(8):1167-1169.
[19]Li X,Chu Z,Liu Y,et al.Molecular characterization of microbial populations in full-scale biofilters treating iron,manganese and ammonia containing groundwater in Harbin,China[J].Bioresource Technology,2013,147:234-239.
[20]杨柳,储昭瑞,任玉辉,等.生物滤池同步去除地下水中Fe2+、Mn2+和As(Ⅲ)的试验研究[J].给水排水,2014,40(3):121-124.
[21]Fu J X,Shang J,Zhao Y H.Simultaneous removal of iron,manganese and ammonia from groundwater in single biofilter layer using BAF[J].Advanced Materials Research,2011,183:442-446.
[22]张建林,李相昆,曾辉平,等.高铁高锰微污染地下水的生物同层净化研究[J].中国给水排水,2011,27(21):5-7.
[23]付伟,李金成,叶雪松,等.生物除锰滤层快速启动中营养投加的效果分析[J].青岛理工大学学报,2013,34(5):76-81.
[24]李灿波,王德生,高进仑,等.生物滤池地下水除铁除锰过程中漏锰现象研究[J].供水技术,2012,6(1):16-19.
[25]商俊,傅金祥,赵玉华,等.BAF工艺处理微污染含铁锰地下水试验研究[J].供水技术,2011,5(2):8-11.
[26]Phatai P,Wittayakun J,Chen W H,et al.Removal of manganese(II)and iron(II)from synthetic groundwater using potassium permanganate[J].Desalination and Water Treatment,2014,52(31-33):5942-5951.
[27]赵焱,李冬,李相昆,等.高效生物除铁除锰工程菌MSB-4的特性研究[J].中国给水排水,2009,25(1):40-44.
[28]Hiiob M,Karro E.Iron in the Middle Devonian aquifer system and its removal at voru county water treatment plants,Estonia[J].Estonian Journal of Earth Sciences,2012,61(3):181.
[29]Burke V,Duennbier U,Massmann G.The effect of aeration on the removal of wastewater-derived pharmaceutical residues from groundwater-a laboratory study[J].Water Science&Technology,2012,67(3):658-666.
[30]Dung N T K,Con T H,Cam B D,et al.Investigation of As,Mn and Fe fixation inside the aquifer during groundwater exploitation in the experimental system imitated natural conditions[J].Environmental Geochemistry and Health,2012,34(3):349-354.
[31]李继震.接触氧化除铁除锰机理的探讨[J].中国给水排水,2010,26(18):6-8.
[32]陈旭.接触氧化法除铁的滤料选择[J].中国新技术新产品,2009,(17):64-64.
[33]熊斌,李星,杨艳玲,等.接触氧化/超滤除铁除锰组合工艺的净化效能[J].中国给水排水,2014,30(1):30-33.
[34]汪洋,黄廷林,文刚.地下水中氨氮、铁、锰的同步去除及其相互作用[J].中国给水排水,2014,30(19):32-39.
[35]王娟珍,薛长安,王志勇,等.高锰酸钾应用于地下水除铁锰试验研究与探讨[J].城镇供水,2013(3):78-80.
[36]Ellis D,Bouchard C,Lantagne G.Removal of iron and manganese from groundwater by oxidation and microfiltration[J].Desalination,2000,130(3):255-264.
[37]沈志余,江锐,王颖,等.高锰酸钾除锰方法在水厂生产中的运用[J].供水技术,2014,8(4):18-21.
[38]吴彦志,李雨时.Fenton试剂-石英砂工艺处理高浓度铁锰地下水[J].科技创新导报,2012(9):132-132.
[39]张俊洁,肖利萍.Fenton试剂和锰砂协同处理铁锰矿井废水的研究[J].水资源与水工程学报,2010,21(5):87-89.
[40]赵玉华,陈芳,李艳凤,等.化学氧化法处理高铁锰微污染地下水的实验[J].沈阳建筑大学学报:自然科学版,2012,28(6):1098-1102.
[41]郦丹,余健,张浩江.氯接触氧化过滤去除原水中锰的试验研究[J].工业水处理,2013,33(10):23-26.
[42]崔恒,郑西来,陈蕾,等.二氧化氯-接触催化氧化联合去除水中铁和锰[J].环境工程学报,2014,8(6):2478-2484.
[43]唐玉兰,武利,傅金祥,等.二氧化氯/混凝剂工艺处理含铁水的试验研究[J].供水技术,2010,4(1):14-16.
[44]薛长安,王娟珍,王志勇.次氯酸钠应用于地下水除铁锰试验研究[J].海峡科技与产业,2013(7):60-61.
[45]Kuberis E A,Gorbachov E A.Environmental monitoring and analysis of quality of the Nizhny Novgorod region ground water with the development of the technologies of their filtration[J].Journal of the Geographical Institute Jovan Cvijic,SASA,2014,64(2):177-191.
[46]Lin J L,Huang C,Pan J R,et al.Fouling mitigation of a dead-end microfiltration by mixing-enhanced preoxidation for Fe and Mn removal from groundwater[J].Colloids and Surfaces A:Physicochemical and Engineering Aspects,2013,419:87-93.
[47]李荧,程家迪,刘锐,等.微滤膜处理铁污染地下水的效果及膜污染控制研究[J].中国给水排水,2010,26(1):36-39.
[48]郭绍东,梁恒,陈杰,等.超滤膜组合工艺处理含铁地下水的效能[J].中国给水排水,2014,30(17):5-8.
[49]Rott U,Meyer C,Friedle M.Residue-free removal of arsenic,iron,manganese and ammonia from groundwater[J].Water Supply,2002,2(1):17-24.
[50]狄军贞,马龙,李爱华,等.铁屑+粉煤灰处理含高浓度铁锰氨氮废水试验研究[J].非金属矿,2012,35(4):61-63.
[51]Munter R,Ojaste H,Sutt J.Complexed iron removal from groundwater[J].Journal of Environmental Engineering,2005,131(7):1014-1020.
[52]Piispanen J K,Sallanko J T.Mn(II)removal from groundwater with manganese oxide-coated filter media[J].Journal of Environmental Science and Health Part A,2010,45(13):1732-1740.
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