水中新型污染物的去除工艺研究进展
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摘要
水体新型污染物检出率和检出种类日益增多,其对生态系统所带来的潜在危害进一步加剧了人们对水质安全的担忧。传统水处理工艺对新型污染物的去除效果并不显著,且存在着不确定性。本文介绍了当前国内外对水体新型污染物的去除工艺及其去除效果,如活性炭吸附、高级氧化技术、膜处理工艺、新型环境功能材料及其组合工艺等,并指出这些工艺存在的不足及今后的发展方向,旨在为水体新型污染物的控制与去除技术提供新的参考。
The detection rate and detection species of new pollutants in water are increasing. At the same time, the potential harm to the ecosystem further increased people's concerns about water quality safety. Nevertheless, the traditional water treatment process has no significant effect on the removal of new pollutants, and there is uncertainty. In this paper, we introduce the removal technology of new pollutants in water bodies at home and abroad, such as activated carbon adsorption, advanced oxidation technology, membrane treatment process, new environmental functional materials and their combination technology. The shortcomings and the future development direction of these processes are also pointed out in order to provide a new reference for the control and remove technology of new pollutants in water.
The detection rate and detection species of new pollutants in water are increasing. At the same time, the potential harm to the ecosystem further increased people's concerns about water quality safety. Nevertheless, the traditional water treatment process has no significant effect on the removal of new pollutants, and there is uncertainty. In this paper, we introduce the removal technology of new pollutants in water bodies at home and abroad, such as activated carbon adsorption, advanced oxidation technology, membrane treatment process, new environmental functional materials and their combination technology. The shortcomings and the future development direction of these processes are also pointed out in order to provide a new reference for the control and remove technology of new pollutants in water.
引文
[1]Paterakis N,Chiu T Y,Koh Y K K,et al.The effectiveness of anaerobic digestion in removing estrogens and nonylphenol ethoxylates[J].Journal of Hazardous Materials,2012,199(2):88-95.
[2]Veetil P G P,Nadaraja A V,Bhasi A,et al.Degradation of Triclosan under Aerobic,Anoxic,and Anaerobic Conditions[J].Applied Biochemistry&Biotechnology,2012,167(6):1603-1612.
[3]黄俊,衣俊,程金平.长江口及近海水环境中新型污染物研究进展[J].环境化学,2014,33(9):1484-1494.
[4]Guieysse B,Noir M L,Bo M.Removal of Endocrine Disrupting Compounds Using Molecularly Imprinted Polymers:A Review[C].2009.
[5]吕露,张梦露,王春明,等.3种典型消毒副产物对细菌抗生素抗性的影响[J].环境科学,2015(7):2525-2531.
[6]刘晶靓.滇池鱼类典型环境内分泌干扰物生物富集及毒性效应研究[D].昆明理工大学,2012.
[7]Petrie B,Barden R,Kasprzyk-Hordern B.A review on emerging contaminants in wastewaters and the environment:current knowledge,understudied areas and recommendations for future monitoring[J].Water Research,2015,72:3-27.
[8]李雪晴.粉末活性碳加强型膜生物反应器对污水中新型污染物的去除[J].水处理技术,2017(12):19-22.
[9]Bernabeu A,Vercher R F,Santos-Juanes L,et al.Solar photocatalysis as a tertiary treatment to remove emerging pollutants from wastewater treatment plant effluents[J].Catalysis Today.2011,161(1):235-240.
[10]Fukuhara T,Iwasaki S,Kawashima M,et al.Adsorbability of estrone and17β-estradiol in water onto activated carbon[J].Water Research.2006,40(2):241.
[11]武睿.活性炭和膜技术去除水中内分泌干扰物的研究进展[J].工业水处理.2010,30(7):11-14.
[12]Pi Y,Feng J,Sun J,et al.Facile,effective,and environment-friendly degradation of sulfamonomethoxine in aqueous solution with the aid of a UV/Oxone oxidative process[J].Environmental Science&Pollution Research International,2013,20(12):8621-8628.
[13]焦宁,宋小康,沈耀良.MBR去除水中新型微污染物PPCPs的效果及影响因素[J].环境工程,2012,30(1):25-29.
[14]周传龙,代朝猛,张亚雷,等.新型环境功能材料去除水体痕量污染物的研究进展[J].材料导报,2012,26(13):145-149.
[15]Cong M,Yu S,Shi W,et al.Effect of different temperatures on performance and membrane fouling in high concentration PAC–MBR system treating micro-polluted surface water[J].Bioresource Technology,2013,141(4):19.
[16]Ma C,Yu S,Shi W,et al.High concentration powdered activated carbon-membrane bioreactor(PAC-MBR)for slightly polluted surface water treatment at low temperature[J].Bioresource Technology,2012,113(2):136-142.
[17]Asada T,Oikawa K,Kawata K,et al.Study of Removal Effect of Bisphenol A andβ-Estradiol by Porous Carbon[J].Journal of Health Science.2004,50(6):588-593.
[18]Adams C,Asce M,Wang Y,et al.Removal of Antibiotics from Surface and Distilled Water in Conventional Water Treatment Processes[J].Journal of Environmental Engineering,2002,128(3):253-260.
[19]Yin C Y,Aroua M K,Wan M A W D.Review of modifications of activated carbon for enhancing contaminant uptakes from aqueous solutions[J].Separation&Purification Technology,2007,52(3):403-415.
[20]刘桂芳.表面改性活性炭吸附酚类内分泌干扰物的性能与机理研究[D].哈尔滨工业大学,2008.
[21]刘桂芳,马军,关春雨,等.改性活性炭对水溶液中双酚-A的吸附研究[J].环境科学,2008,29(2):349-355.
[22]Fukuhara T,Iwasaki S,Kawashima M,et al.Adsorbability of estrone and17β-estradiol in water onto activated carbon[J].Water Research,2006,40(2):241.
[23]Broséus R,Vincent S,Aboulfadl K,et al.Ozone oxidation of pharmaceuticals,endocrine disruptors and pesticides during drinking water treatment[J].Water Research,2009,43(18):4707.
[24]王翠彦,李梅,王洪波,等.光催化氧化去除水中新型有机污染物研究进展[J].山东建筑大学学报,2012,27(4):426-430.
[25]Lin J J,Zhao X S,Liu D,et al.The decoloration and mineralization of azo dye C.I.Acid Red 14 by sonochemical process:Rate improvement via Fenton's reactions[J].Journal of Hazardous Materials,2008,157(2-3):541-546.
[26]黄金鑫,杨海,李海峰,等.电化学氧化还原法降解卤代有机污染物的研究进展[J].化学试剂.2017(1):29-36.
[27]Huber M M,Canonica S,Park G Y,et al.Oxidation of pharmaceuticals during ozonation and advanced oxidation processes[J].Environmental Science&Technology,2003,37(5):1016-1024.
[28]Chatzitakis A,Berberidou C,Paspaltsis I,et al.Photocatalytic degradation and drug activity reduction of Chloramphenicol[J].Water Research,2008,42(1):386-394.
[29]Marinas A,Guillard C,Marinas J M,et al.Photocatalytic degradation of pesticide–acaricide formetanate in aqueous suspension of Ti O[J].Applied Catalysis B Environmental,2001,34(3):241-252.
[30]Hamdaoui O,Chiha M,Naffrechoux E.Ultrasound-assisted removal of malachite green from aqueous solution by dead pine needles[J].Ultrasonics Sonochemistry,2008,15(5):799-807.
[31]胡俊生,徐志荣,李春荣,等.水体中对氯苯酚的电化学降解研究[J].沈阳建筑大学学报(自然科学版),2007,23(5):822-825.
[32]Park J,Quaiserová-Mocko V,PeckováK,et al.Fabrication,characterization,and application of a diamond microelectrode for electrochemical measurement of norepinephrine release from the sympathetic nervous system[J].Diamond&Related Materials,2006,15(4-8):761-772.
[33]Fatta-Kassinos D,Dionysiou D D,Kümmerer K.Advanced Treatment Technologies for Urban Wastewater Reuse[M].Springer International Publishing,2016.
[34]Sun B,Guan X,Fang J,et al.Activation of Manganese Oxidants with Bisulfite for Enhanced Oxidation of Organic Contaminants:The Involvement of Mn(III)[J].Environmental Science&Technology,2015,49(20):12414-12421.
[35]皮运清.高级氧化技术对典型PPCPs降解效果及降解机理的研究[D].河南师范大学,2013.
[36]李圭白,张杰.水质工程学[M].中国建筑工业出版社,2013.
[37]Sipma J,Osuna B,Collado N,et al.Comparison of removal of pharmaceuticals in MBR and activated sludge systems☆[J].Desalination,2010,250(2):653-659.
[38]Urase T,Kagawa C,Kikuta T.Factors affecting removal of pharmaceutical substances and estrogens in membrane separation bioreactors[J].Desalination,2004,178(1):107-113.
[39]Mansell B,Kuo J,Tang C C,et al.EVALUATION OF REMOVALS OF NDMA,HORMONES,PHARMACEUTICALS,AND PERSONAL CARE PRODUCTS IN A MEMBRANE BIOREACTOR[J].Proceedings of the Water Environment Federation,2005:7411-7427.
[40]Acero J L,Benitez F J,Teva F,et al.Retention of emerging micropollutants from UP water and a municipal secondary effluent by ultrafiltration and nanofiltration[J].Chemical Engineering Journal,2010,163(3):264-272.
[41]Siegrist H,Joss A.Review on the fate of organic micropollutants in wastewater treatment and water reuse with membranes[J].Water Science&Technology A Journal of the International Association on Water Pollution Research,2012,66(6):1369.
[42]Judd S J.Membrane technology costs and me[J].Water Research,2017,122:1.
[43]Meng F,Zhang S,Oh Y,et al.Fouling in membrane bioreactors:An updated review[J].Water Research,2017,114:151.
[44]Meng F,Zhou Z,Ni B J,et al.Characterization of the size-fractionated biomacromolecules:Tracking their role and fate in a membrane bioreactor[J].Water Research,2011,45(15):4661-4671.
[45]周传龙,代朝猛,张亚雷,等.新型环境功能材料去除水体痕量污染物的研究进展[J].材料导报,2012,26(13):145-149.
[46]Zhang L,Song X,Liu X,et al.Studies on the removal of tetracycline by multi-walled carbon nanotubes[J].Chemical Engineering Journal,2011,178(24):26-33.
[47]Cui X,Yang S,Yan X,et al.Pyridinic-Nitrogen-Dominated Graphene Aerogels with Fe-N-C Coordination for Highly Efficient Oxygen Reduction Reaction[J].Advanced Functional Materials,2016,26(31):5708-5717.
[48]Yao Y,Lian C,Wu G,et al.Synthesis of“Sea Urchin”-like Carbon Nanotubes/Porous Carbon Superstructures Derived from Waste Biomass for Treatment of Various Contaminants[J].Applied Catalysis B Environmental,2017,219.
[49]Martucci A,Cremonini M A,Blasioli S,et al.Adsorption and reaction of sulfachloropyridazine sulfonamide antibiotic on a high silica mordenite:A structural and spectroscopic combined study[J].Microporous&Mesoporous Materials,2013,170(2):274-286.
[50]Noir M L,Plieva F,Bo M.Removal of Endocrine Disrupting Contaminants from Water Using Macroporous Molecularly Imprinted Selective Media[J].Acs Symposium,2009,1022:25-51.
[51]Dai C M,Geissen S U,Zhang Y L,et al.Performance evaluation and application of molecularly imprinted polymer for separation of carbamazepine in aqueous solution[J].Journal of Hazardous Materials,2010,184(1-3):156-163.
[52]Yanghsin S,Tai Y T.Reaction of decabrominated diphenyl ether by zerovalent iron nanoparticles[J].Chemosphere,2010,78(10):1200-1206.
[53]Wiesner M R,Lowry G V,Alvarez P,et al.Assessing the Risks of Manufactured Nanomaterials[J].Environmental Science&Technology,2006,40(14):4336-4345.
[54]高燕飞,高乃云.纳米铁及其改性材料在水处理中的应用[J].给水排水,2011,37(1):108-113.
[55]马聪.粉末活性炭/膜组合工艺处理低温微污染水的效能[D].哈尔滨工业大学,2013.
[56]乔铁军.活性炭—超滤复合工艺去除水中典型PPCPs的效能与机理[D].清华大学,2011.
[57]黄瑾辉,曾光明,刘萍,等.颗粒活性炭-超滤膜联用工艺去除管网水中微量有机物[J].水处理技术,2007,33(1):74-78.
[58]Jegatheesan V,Senaratne N,Steicke C,et al.Powdered activated carbon for fouling reduction of a membrane in a pilot-scale recirculating aquaculture system[J].Desalination&Water Treatment,2009,5(1-3):1-5.
[59]Satyawali Y,Balakrishnan M.Performance enhancement with powdered activated carbon(PAC)addition in a membrane bioreactor(MBR)treating distillery effluent.[J].Journal of Hazardous Materials,2009,170(1):457-465.
[60]张瑞金,陈鑫,邓慧萍,等.附加电场超滤膜去除水中有机污染物的研究[J].工业水处理,2012,32(4):24-28.
[2]Veetil P G P,Nadaraja A V,Bhasi A,et al.Degradation of Triclosan under Aerobic,Anoxic,and Anaerobic Conditions[J].Applied Biochemistry&Biotechnology,2012,167(6):1603-1612.
[3]黄俊,衣俊,程金平.长江口及近海水环境中新型污染物研究进展[J].环境化学,2014,33(9):1484-1494.
[4]Guieysse B,Noir M L,Bo M.Removal of Endocrine Disrupting Compounds Using Molecularly Imprinted Polymers:A Review[C].2009.
[5]吕露,张梦露,王春明,等.3种典型消毒副产物对细菌抗生素抗性的影响[J].环境科学,2015(7):2525-2531.
[6]刘晶靓.滇池鱼类典型环境内分泌干扰物生物富集及毒性效应研究[D].昆明理工大学,2012.
[7]Petrie B,Barden R,Kasprzyk-Hordern B.A review on emerging contaminants in wastewaters and the environment:current knowledge,understudied areas and recommendations for future monitoring[J].Water Research,2015,72:3-27.
[8]李雪晴.粉末活性碳加强型膜生物反应器对污水中新型污染物的去除[J].水处理技术,2017(12):19-22.
[9]Bernabeu A,Vercher R F,Santos-Juanes L,et al.Solar photocatalysis as a tertiary treatment to remove emerging pollutants from wastewater treatment plant effluents[J].Catalysis Today.2011,161(1):235-240.
[10]Fukuhara T,Iwasaki S,Kawashima M,et al.Adsorbability of estrone and17β-estradiol in water onto activated carbon[J].Water Research.2006,40(2):241.
[11]武睿.活性炭和膜技术去除水中内分泌干扰物的研究进展[J].工业水处理.2010,30(7):11-14.
[12]Pi Y,Feng J,Sun J,et al.Facile,effective,and environment-friendly degradation of sulfamonomethoxine in aqueous solution with the aid of a UV/Oxone oxidative process[J].Environmental Science&Pollution Research International,2013,20(12):8621-8628.
[13]焦宁,宋小康,沈耀良.MBR去除水中新型微污染物PPCPs的效果及影响因素[J].环境工程,2012,30(1):25-29.
[14]周传龙,代朝猛,张亚雷,等.新型环境功能材料去除水体痕量污染物的研究进展[J].材料导报,2012,26(13):145-149.
[15]Cong M,Yu S,Shi W,et al.Effect of different temperatures on performance and membrane fouling in high concentration PAC–MBR system treating micro-polluted surface water[J].Bioresource Technology,2013,141(4):19.
[16]Ma C,Yu S,Shi W,et al.High concentration powdered activated carbon-membrane bioreactor(PAC-MBR)for slightly polluted surface water treatment at low temperature[J].Bioresource Technology,2012,113(2):136-142.
[17]Asada T,Oikawa K,Kawata K,et al.Study of Removal Effect of Bisphenol A andβ-Estradiol by Porous Carbon[J].Journal of Health Science.2004,50(6):588-593.
[18]Adams C,Asce M,Wang Y,et al.Removal of Antibiotics from Surface and Distilled Water in Conventional Water Treatment Processes[J].Journal of Environmental Engineering,2002,128(3):253-260.
[19]Yin C Y,Aroua M K,Wan M A W D.Review of modifications of activated carbon for enhancing contaminant uptakes from aqueous solutions[J].Separation&Purification Technology,2007,52(3):403-415.
[20]刘桂芳.表面改性活性炭吸附酚类内分泌干扰物的性能与机理研究[D].哈尔滨工业大学,2008.
[21]刘桂芳,马军,关春雨,等.改性活性炭对水溶液中双酚-A的吸附研究[J].环境科学,2008,29(2):349-355.
[22]Fukuhara T,Iwasaki S,Kawashima M,et al.Adsorbability of estrone and17β-estradiol in water onto activated carbon[J].Water Research,2006,40(2):241.
[23]Broséus R,Vincent S,Aboulfadl K,et al.Ozone oxidation of pharmaceuticals,endocrine disruptors and pesticides during drinking water treatment[J].Water Research,2009,43(18):4707.
[24]王翠彦,李梅,王洪波,等.光催化氧化去除水中新型有机污染物研究进展[J].山东建筑大学学报,2012,27(4):426-430.
[25]Lin J J,Zhao X S,Liu D,et al.The decoloration and mineralization of azo dye C.I.Acid Red 14 by sonochemical process:Rate improvement via Fenton's reactions[J].Journal of Hazardous Materials,2008,157(2-3):541-546.
[26]黄金鑫,杨海,李海峰,等.电化学氧化还原法降解卤代有机污染物的研究进展[J].化学试剂.2017(1):29-36.
[27]Huber M M,Canonica S,Park G Y,et al.Oxidation of pharmaceuticals during ozonation and advanced oxidation processes[J].Environmental Science&Technology,2003,37(5):1016-1024.
[28]Chatzitakis A,Berberidou C,Paspaltsis I,et al.Photocatalytic degradation and drug activity reduction of Chloramphenicol[J].Water Research,2008,42(1):386-394.
[29]Marinas A,Guillard C,Marinas J M,et al.Photocatalytic degradation of pesticide–acaricide formetanate in aqueous suspension of Ti O[J].Applied Catalysis B Environmental,2001,34(3):241-252.
[30]Hamdaoui O,Chiha M,Naffrechoux E.Ultrasound-assisted removal of malachite green from aqueous solution by dead pine needles[J].Ultrasonics Sonochemistry,2008,15(5):799-807.
[31]胡俊生,徐志荣,李春荣,等.水体中对氯苯酚的电化学降解研究[J].沈阳建筑大学学报(自然科学版),2007,23(5):822-825.
[32]Park J,Quaiserová-Mocko V,PeckováK,et al.Fabrication,characterization,and application of a diamond microelectrode for electrochemical measurement of norepinephrine release from the sympathetic nervous system[J].Diamond&Related Materials,2006,15(4-8):761-772.
[33]Fatta-Kassinos D,Dionysiou D D,Kümmerer K.Advanced Treatment Technologies for Urban Wastewater Reuse[M].Springer International Publishing,2016.
[34]Sun B,Guan X,Fang J,et al.Activation of Manganese Oxidants with Bisulfite for Enhanced Oxidation of Organic Contaminants:The Involvement of Mn(III)[J].Environmental Science&Technology,2015,49(20):12414-12421.
[35]皮运清.高级氧化技术对典型PPCPs降解效果及降解机理的研究[D].河南师范大学,2013.
[36]李圭白,张杰.水质工程学[M].中国建筑工业出版社,2013.
[37]Sipma J,Osuna B,Collado N,et al.Comparison of removal of pharmaceuticals in MBR and activated sludge systems☆[J].Desalination,2010,250(2):653-659.
[38]Urase T,Kagawa C,Kikuta T.Factors affecting removal of pharmaceutical substances and estrogens in membrane separation bioreactors[J].Desalination,2004,178(1):107-113.
[39]Mansell B,Kuo J,Tang C C,et al.EVALUATION OF REMOVALS OF NDMA,HORMONES,PHARMACEUTICALS,AND PERSONAL CARE PRODUCTS IN A MEMBRANE BIOREACTOR[J].Proceedings of the Water Environment Federation,2005:7411-7427.
[40]Acero J L,Benitez F J,Teva F,et al.Retention of emerging micropollutants from UP water and a municipal secondary effluent by ultrafiltration and nanofiltration[J].Chemical Engineering Journal,2010,163(3):264-272.
[41]Siegrist H,Joss A.Review on the fate of organic micropollutants in wastewater treatment and water reuse with membranes[J].Water Science&Technology A Journal of the International Association on Water Pollution Research,2012,66(6):1369.
[42]Judd S J.Membrane technology costs and me[J].Water Research,2017,122:1.
[43]Meng F,Zhang S,Oh Y,et al.Fouling in membrane bioreactors:An updated review[J].Water Research,2017,114:151.
[44]Meng F,Zhou Z,Ni B J,et al.Characterization of the size-fractionated biomacromolecules:Tracking their role and fate in a membrane bioreactor[J].Water Research,2011,45(15):4661-4671.
[45]周传龙,代朝猛,张亚雷,等.新型环境功能材料去除水体痕量污染物的研究进展[J].材料导报,2012,26(13):145-149.
[46]Zhang L,Song X,Liu X,et al.Studies on the removal of tetracycline by multi-walled carbon nanotubes[J].Chemical Engineering Journal,2011,178(24):26-33.
[47]Cui X,Yang S,Yan X,et al.Pyridinic-Nitrogen-Dominated Graphene Aerogels with Fe-N-C Coordination for Highly Efficient Oxygen Reduction Reaction[J].Advanced Functional Materials,2016,26(31):5708-5717.
[48]Yao Y,Lian C,Wu G,et al.Synthesis of“Sea Urchin”-like Carbon Nanotubes/Porous Carbon Superstructures Derived from Waste Biomass for Treatment of Various Contaminants[J].Applied Catalysis B Environmental,2017,219.
[49]Martucci A,Cremonini M A,Blasioli S,et al.Adsorption and reaction of sulfachloropyridazine sulfonamide antibiotic on a high silica mordenite:A structural and spectroscopic combined study[J].Microporous&Mesoporous Materials,2013,170(2):274-286.
[50]Noir M L,Plieva F,Bo M.Removal of Endocrine Disrupting Contaminants from Water Using Macroporous Molecularly Imprinted Selective Media[J].Acs Symposium,2009,1022:25-51.
[51]Dai C M,Geissen S U,Zhang Y L,et al.Performance evaluation and application of molecularly imprinted polymer for separation of carbamazepine in aqueous solution[J].Journal of Hazardous Materials,2010,184(1-3):156-163.
[52]Yanghsin S,Tai Y T.Reaction of decabrominated diphenyl ether by zerovalent iron nanoparticles[J].Chemosphere,2010,78(10):1200-1206.
[53]Wiesner M R,Lowry G V,Alvarez P,et al.Assessing the Risks of Manufactured Nanomaterials[J].Environmental Science&Technology,2006,40(14):4336-4345.
[54]高燕飞,高乃云.纳米铁及其改性材料在水处理中的应用[J].给水排水,2011,37(1):108-113.
[55]马聪.粉末活性炭/膜组合工艺处理低温微污染水的效能[D].哈尔滨工业大学,2013.
[56]乔铁军.活性炭—超滤复合工艺去除水中典型PPCPs的效能与机理[D].清华大学,2011.
[57]黄瑾辉,曾光明,刘萍,等.颗粒活性炭-超滤膜联用工艺去除管网水中微量有机物[J].水处理技术,2007,33(1):74-78.
[58]Jegatheesan V,Senaratne N,Steicke C,et al.Powdered activated carbon for fouling reduction of a membrane in a pilot-scale recirculating aquaculture system[J].Desalination&Water Treatment,2009,5(1-3):1-5.
[59]Satyawali Y,Balakrishnan M.Performance enhancement with powdered activated carbon(PAC)addition in a membrane bioreactor(MBR)treating distillery effluent.[J].Journal of Hazardous Materials,2009,170(1):457-465.
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