垃圾渗滤液尾水氮的深度处理技术研究进展
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摘要
根据垃圾渗滤液尾水特点,系统分析了现有工艺的优缺点,认为物化处理技术不能实现垃圾渗滤液尾水的完全脱氮,但可作为前处理或辅助手段,而生物法是实现氮脱除的经济有效方法,但需要结合填埋场特点考虑电子供体来源。同时,提出了一种脱氮工艺——硫铁自养反硝化工艺,并进行了可行性分析。
According to the characteristics of the tail water of landfill leachate,the advantages and disadvantages of the existing process were systematically analyzed.It was considered that the physical and chemical treatment technology could not realize the complete denitrification of the tail water of landfill leachate,but it could be used as a pretreatment or auxiliary method.And the biological method was economical and efficient to realize nitrogen removal,but it was necessary to consider the source of the electron donor with the characteristics of the landfill.At the same time,a S/Fe autotrophic denitrification process was proposed and feasibility analysis was carried out.
According to the characteristics of the tail water of landfill leachate,the advantages and disadvantages of the existing process were systematically analyzed.It was considered that the physical and chemical treatment technology could not realize the complete denitrification of the tail water of landfill leachate,but it could be used as a pretreatment or auxiliary method.And the biological method was economical and efficient to realize nitrogen removal,but it was necessary to consider the source of the electron donor with the characteristics of the landfill.At the same time,a S/Fe autotrophic denitrification process was proposed and feasibility analysis was carried out.
引文
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[23]李文龙,杨碧印,陈益清,等.不同外加碳源反硝化滤池的深度脱氮特性研究[J].水处理技术,2015,41(11):82-85.
[24]郭炜.臭氧氧化-曝气生物滤池联合工艺深度处理垃圾渗滤液的应用研究[J].广东化工,2017,44(11):224-225.
[25]张永森,郑彤,孙彦龙,等.臭氧-活性炭组合工艺深度处理垃圾渗滤液MBR出水[J].环境工程学报,2017,11(8):4535-4541.
[26] REMMAS N,MELIDIS P,KATSIOUPI E,et al.Effects of high organic load on amoA and nirS gene diversity of an intermittently aerated and fed membrane bioreactor treating landfill leachate[J].Bioresource Technology,2016,220:557-565.
[27]任琦,张占东.外加碳源处理低C/N污水研究现状[J].科技风,2018(14):119.
[28]马勇,彭永臻,王淑莹.不同外碳源对污泥反硝化特性的影响[J].北京工业大学学报,2009,35(6):820-824.
[29] WANG J,CHU L.Biological nitrate removal from water and wastewater by solid-phase denitrification process[J].Biotechnology Advances,2016,34(6).
[30]朱擎,杨飞飞,赵兰,等.两种共混BDPs作为生物膜载体和碳源的脱氮研究比较[J].北京大学学报(自然科学版),2015,51(3):525-530.
[31] LI P,ZUO J,WANG Y,et al.Tertiary nitrogen removal for municipal wastewater using a solid-phase denitrifying biofilter with polycaprolactone as the carbon source and filtration medium[J].Water Research,2016,93:74-83.
[32] GAO H,HE J,WANG Y,et al.Advantageous combination of solid carbon paste and a conducting polymer film as a support of platinum electrocatalyst for methanol fuel cell[J].Journal of Power Sources,2012,205(2):164-172.
[33] YANG X,JIANG Q,SONG H,et al.Selection and application of agricultural wastes as solid carbon sources and biofilm carriers in MBR[J].Journal of Hazardous Materials,2015,283:186-192.
[34] ZHANG S,SUN X,FAN Y,et al.Heterotrophic nitrification and aerobic denitrification by Diaphorobacter polyhydroxybutyrativorans SL-205 using poly(3-hydroxybutyrate-co-3-hydroxyvalerate)as the sole carbon source[J].Bioresource Technology,2017,241:500-507.
[35] CHU L,WANG J.Denitrification performance and biofilm characteristics using biodegradable polymers PCL as carriers and carbon source[J].Chemosphere,2013,91(9):1310-1316.
[36] YAN F,JIANG J,ZHANG H,et al.denitrification from mature landfill leachate using a food-waste-derived carbon source[J].Journal of Environmental Management,2018,214:184-191.
[37] KARANASIOS K A,VASILIADOU I A,PAVLOU S,et al.Hydrogenotrophic denitrification of potable water:a review[J].Journal of Hazardous Materials,2010,180(1):20-37.
[38] LEE K C,RITTMANN B E.Applying a novel autohydrogenotrophic hollow-fiber membrane biofilm reactor for denitrification of drinking water[J].Water Research,2002,36(8):2040-2052.
[39]王振兴,李向全,侯新伟,等.地下水硝酸盐污染的生物修复技术研究进展[J].环境科学与技术,2012,35(增刊1):163-166.
[40]王弘宇,张惠宁,吕斌,等.铁基质自养反硝化去除水中硝酸盐污染物的研究[J].中国农村水利水电,2014(11):59-62.
[41]彭彬,刘燕,张旭栋.铁刨花对上流式厌氧污泥床反应器室温下处理城镇污水的影响[J].复旦学报(自然科学版),2008,47(3):398-402.
[42] RIVETT M O,BUSS S R,MORGAN P,et al.Nitrate attenuation in groundwater:a review of biogeochemical controlling processes[J].Water Research,2008,42(16):4215-4232.
[43]李天昕,邱诚翔,徐昊,等.硫/石灰石自养反硝化处理低碳高氮城市污水的工艺[J].环境工程学报,2014,8(3):1062-1066.
[44]任争鸣,刘雪洁,苏晓磊,等.硫自养反硝化深度脱氮中试研究[J].中国给水排水,2016,32(19):31-35.
[45] WAN T,ZHANG G,DU F,et al.Combined biologic aerated filter and sulfur/ceramisite autotrophic denitrification for advanced wastewater nitrogen removal at low temperatures[J].Higher Education Press,2014,8(6):967-972.
[46]袁莹,周伟丽,王晖,等.不同电子供体的硫自养反硝化脱氮实验研究[J].环境科学,2013,34(5):1835-1844.
[47] CHUNG J,AMIN K,KIM S,et al.Autotrophic denitrification of nitrate and nitrite using thiosulfate as an electron donor[J].Water Research,2014,58(3):169-178.
[48]陈建军,张建,黄民生,等.硝酸盐介导底泥硫自养反硝化的过程、效应和应用[J].华东师范大学学报(自然科学版),2015(2):91-97.
[49]支尧,张光生,钱凯,等.生物吸附/MBR/硫铁自养反硝化组合工艺优化研究[J].中国环境科学,2018,38(6):2097-2104.
[50]霍珊.基于S—Fe氧化的自养反硝去除水中NO3--N的研究[D].北京:北京化工大学,2016.
[2] ZHOU L,ZHUANG W,YE B,et al.Inorganic characteristics of cake layer in A/O MBR for anaerobically digested leachate from municipal solid waste incineration plant with MAP pretreatment[J].Chemical Engineering Journal,2017,327:71-78.
[3] YONG Z J,BASHIR M J K,NG C A,et al.A sequential treatment of intermediate tropical landfill leachate using a sequencing batch reactor(SBR)and coagulation[J].Journal of Environmental Management,2018,205:244-252.
[4] CHEN Z,WANG X,YANG Y,et al.Partial nitrification and denitrification of mature landfill leachate using apilot-scale continuous activated sludge process at low dissolved oxygen[J].Bioresource Technology,2016,218:580-588.
[5]胡学斌,杨柳,吉芳英,等.低碳源城市污水的低氧同步脱氮除磷研究[J].中国给水排水,2009,25(13):16-19.
[6]曹贵华,黄勇,潘杨.常规生物脱氮除磷工艺中问题及对策[J].水处理技术,2009,35(3):102-106.
[7]孙永利,许光明,游佳,等.城镇污水处理厂外加商业碳源的选择[J].中国给水排水,2010,26(19):84-86.
[8] WU L,ZHANG L,SHI X,et al.Analysis of the impact of reflux ratio on coupled partial nitrification-anammox for co-treatment of mature landfill leachate and domestic wastewater[J].Bioresource Technology,2015,198:207-214.
[9]张瑛,阮晓红.水处理混凝剂及其发展方向[J].污染防治技术,2003,16(4):45-49.
[10]宋相松.吸附剂与混凝剂联合应用于再生水除氮的实验研究[D].郑州:华北水利水电大学,2016.
[11]张勇.三维电极深度处理渗滤液混凝出水的定性研究[J].山西化工,2016,36(3):95-98.
[12]唐国卿.臭氧高级氧化应用于垃圾渗滤液NF浓缩液工程中总氮的去除的案例[J].环境与发展,2017,29(10).
[13] HASAR H,UNSAL S A,IPEK U,et al.Stripping/flocculation/membrane bioreactor/reverse osmosis treatment of municipal landfill leachate[J].Journal of Hazardous Materials,2009,171(1):309-317.
[14] SR M,PODHOLA M,PATOˇCKA T,et al.The effect of humic acids on the reverse osmosis treatment of hazardous landfill leachate[J].Journal of Hazardous Materials,2012,207/208:86-90.
[15] OZTURK I,ALTINBAS M,KOYUNCU I,et al.Advanced physico-chemical treatment experiences on young municipal landfill leachates[J].Waste Management,2003,23(5):441-446.
[16] BRUGGEN B V D,EVERAERT K,WILMS D,et al.Application of nanofiltration for removal of pesticides,nitrate and hardness from ground water:rejection properties and economic evaluation[J].Journal of Membrane Science,2001,193(2):239-248.
[17]延利军.水中硝酸盐污染现状、危害及脱除技术[J].能源环境保护,2013,27(3):39-42.
[18]郑敏.铁碳微电解对垃圾渗滤液生化出水水质改善研究[D].哈尔滨:哈尔滨工业大学,2017.
[19] SAKKAS V,CALZA P,AZHARUL ISLAM M,et al.TiO2/H2O2 mediated photocatalytic transformation of UV filter4-methylbenzylidene camphor(4-MBC)in aqueous phase:statistical optimization and photoproduct analysis[J].Applied Catalysis B:Environmental,2009,90(3):526-534.
[20]孙洋.垃圾渗滤液光化学组合工艺试验研究与装置研发[D].南昌:南昌大学,2017.
[21]史朝霞.不同类型生物反应器填埋场氮污染物转化特性研究[D].成都:西南交通大学,2017.
[22]胡香,张辉,许光远,等.反硝化深床滤池深度脱氮效果研究[J].中国给水排水,2017,33(21):13-17.
[23]李文龙,杨碧印,陈益清,等.不同外加碳源反硝化滤池的深度脱氮特性研究[J].水处理技术,2015,41(11):82-85.
[24]郭炜.臭氧氧化-曝气生物滤池联合工艺深度处理垃圾渗滤液的应用研究[J].广东化工,2017,44(11):224-225.
[25]张永森,郑彤,孙彦龙,等.臭氧-活性炭组合工艺深度处理垃圾渗滤液MBR出水[J].环境工程学报,2017,11(8):4535-4541.
[26] REMMAS N,MELIDIS P,KATSIOUPI E,et al.Effects of high organic load on amoA and nirS gene diversity of an intermittently aerated and fed membrane bioreactor treating landfill leachate[J].Bioresource Technology,2016,220:557-565.
[27]任琦,张占东.外加碳源处理低C/N污水研究现状[J].科技风,2018(14):119.
[28]马勇,彭永臻,王淑莹.不同外碳源对污泥反硝化特性的影响[J].北京工业大学学报,2009,35(6):820-824.
[29] WANG J,CHU L.Biological nitrate removal from water and wastewater by solid-phase denitrification process[J].Biotechnology Advances,2016,34(6).
[30]朱擎,杨飞飞,赵兰,等.两种共混BDPs作为生物膜载体和碳源的脱氮研究比较[J].北京大学学报(自然科学版),2015,51(3):525-530.
[31] LI P,ZUO J,WANG Y,et al.Tertiary nitrogen removal for municipal wastewater using a solid-phase denitrifying biofilter with polycaprolactone as the carbon source and filtration medium[J].Water Research,2016,93:74-83.
[32] GAO H,HE J,WANG Y,et al.Advantageous combination of solid carbon paste and a conducting polymer film as a support of platinum electrocatalyst for methanol fuel cell[J].Journal of Power Sources,2012,205(2):164-172.
[33] YANG X,JIANG Q,SONG H,et al.Selection and application of agricultural wastes as solid carbon sources and biofilm carriers in MBR[J].Journal of Hazardous Materials,2015,283:186-192.
[34] ZHANG S,SUN X,FAN Y,et al.Heterotrophic nitrification and aerobic denitrification by Diaphorobacter polyhydroxybutyrativorans SL-205 using poly(3-hydroxybutyrate-co-3-hydroxyvalerate)as the sole carbon source[J].Bioresource Technology,2017,241:500-507.
[35] CHU L,WANG J.Denitrification performance and biofilm characteristics using biodegradable polymers PCL as carriers and carbon source[J].Chemosphere,2013,91(9):1310-1316.
[36] YAN F,JIANG J,ZHANG H,et al.denitrification from mature landfill leachate using a food-waste-derived carbon source[J].Journal of Environmental Management,2018,214:184-191.
[37] KARANASIOS K A,VASILIADOU I A,PAVLOU S,et al.Hydrogenotrophic denitrification of potable water:a review[J].Journal of Hazardous Materials,2010,180(1):20-37.
[38] LEE K C,RITTMANN B E.Applying a novel autohydrogenotrophic hollow-fiber membrane biofilm reactor for denitrification of drinking water[J].Water Research,2002,36(8):2040-2052.
[39]王振兴,李向全,侯新伟,等.地下水硝酸盐污染的生物修复技术研究进展[J].环境科学与技术,2012,35(增刊1):163-166.
[40]王弘宇,张惠宁,吕斌,等.铁基质自养反硝化去除水中硝酸盐污染物的研究[J].中国农村水利水电,2014(11):59-62.
[41]彭彬,刘燕,张旭栋.铁刨花对上流式厌氧污泥床反应器室温下处理城镇污水的影响[J].复旦学报(自然科学版),2008,47(3):398-402.
[42] RIVETT M O,BUSS S R,MORGAN P,et al.Nitrate attenuation in groundwater:a review of biogeochemical controlling processes[J].Water Research,2008,42(16):4215-4232.
[43]李天昕,邱诚翔,徐昊,等.硫/石灰石自养反硝化处理低碳高氮城市污水的工艺[J].环境工程学报,2014,8(3):1062-1066.
[44]任争鸣,刘雪洁,苏晓磊,等.硫自养反硝化深度脱氮中试研究[J].中国给水排水,2016,32(19):31-35.
[45] WAN T,ZHANG G,DU F,et al.Combined biologic aerated filter and sulfur/ceramisite autotrophic denitrification for advanced wastewater nitrogen removal at low temperatures[J].Higher Education Press,2014,8(6):967-972.
[46]袁莹,周伟丽,王晖,等.不同电子供体的硫自养反硝化脱氮实验研究[J].环境科学,2013,34(5):1835-1844.
[47] CHUNG J,AMIN K,KIM S,et al.Autotrophic denitrification of nitrate and nitrite using thiosulfate as an electron donor[J].Water Research,2014,58(3):169-178.
[48]陈建军,张建,黄民生,等.硝酸盐介导底泥硫自养反硝化的过程、效应和应用[J].华东师范大学学报(自然科学版),2015(2):91-97.
[49]支尧,张光生,钱凯,等.生物吸附/MBR/硫铁自养反硝化组合工艺优化研究[J].中国环境科学,2018,38(6):2097-2104.
[50]霍珊.基于S—Fe氧化的自养反硝去除水中NO3--N的研究[D].北京:北京化工大学,2016.
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