摘要
碳纳米粒子悬浮液具有良好的光限幅性质,是一种优良的宽波段光限幅材料。通过热传导方程和米氏散射理论建立了微气泡半径与入射光能量、碳纳米粒子悬浮液散射系数和透过率的理论模型。采用Matlab数值模拟了散射系数随微气泡尺寸因子的变化关系,碳纳米粒子悬浮液光限幅性能随入射光能量的变化规律。研究了气泡尺寸因子、入射激光能量以及波长对碳纳米粒子悬浮液光限幅特性的影响。研究发现当激光能量达到一定值时,微气泡的半径保持恒定,不再随入射激光能量的增加而增加。微气泡尺寸的增大对碳纳米粒子悬浮液的透过率有着显著的影响。同时,碳纳米粒子悬浮液对不同入射光波长和光能表现出不同的光限幅性能。研究结果为实验研究提供了理论指导。
Carbon nanoparticle suspension has a good optical limiting properties,which is an excellent broadband optical limiting material.The relationship between micro-bubble radius and the incident light energy,theoretical mode of carbon nanoparticles suspension scattering coefficient and transmission ratio are established by heat conduction equations and Mie scattering theory.The variation of the scattering coefficient with the micro bubble size factor and optical limiting properties' change law with the incident light energy's change are simulated by matlab.The effects of bubble size factor,incident laser energy and wavelength on the optical limiting properties of carbon nanoparticles are investigated.It shows that when the laser energy reaches a certain value,the radius of the micro bubbles is kept constant,and no longer increases with the increase of the laser energy.The increase of micro bubble size has a significant effect on the transmittance of the suspensions of carbon nanoparticles.Meanwhile,carbon nanoparticle suspension has different optical limiting properties for different incident light wavelengths and light energy.The research results provide theoretical guidance for the experimental study.
引文
[1]骆永全,王伟平,李剑峰,等.碳纳米管悬浮液的光限幅特性实验研究[J].强激光与粒子束,2006,18(6):895-898.(Luo Yongquan,Wang Weiping,Li Jianfeng,et al.Experiment study on optical limiting properities of carbon nanotube suspensions[J].High Power Laser and Particle Beams,2006,18(6):895-898)
[2]Belousova I M,Mironova N G,Yur’Ev M S.Theoretical investigation of nonlinear limiting of laser radiation power by suspensions of carbon particles[J].Opt Spectrosc,2003,94(1):86-91.
[3]Mishra S R,Rawat H S,Joshi M P,et al.The role of non-linear scattering in optical limiting in C60solutions[J].J Phys B,1994,27(8):L157.
[4]王彩丽,牛燕雄,崔云霞.碳纳米颗粒悬浮液光限幅性能理论分析和数值模拟[J].红外与激光工程,2012,41(5):1186-1190.(Wang Caili,Niu Yanxiong,Cui Yunxia,Theoretical analysis and numerical simulation of optical limiting properties of carbon nanoparticle suspension[J].Infrared and Laser Engineering,2012,41(5):1186-1190)
[5]Belousova I M,Mironova N G,Scobelev A G,et al.The investigation of nonlinear optical limiting by aqueous suspensions of carbon nanoparticles[J].Opt Commun,2004,235(4):445-452.
[6]王亚伟.光散射理论及其应用技术[M].北京:北京科学出版社,2013.28-29.(Wang Yawei,Light scattering theory and its application technology[M].Beijing:Beijing Science Press,2013,28-29)
[7]Mansour K,Soileau M J,Van Stryland E W.Nonlinear optical properties of carbon-black suspensions(ink)[J].JOSA B,1992,9(7):1100-1109.