分子钙钛矿含能材料（英文）
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摘要
设计合成兼具良好爆轰性能、高稳定性和低成本的含能化合物是发展实用含能材料的关键.本文报道了一类新型分子钙钛矿含能化合物,它们可以通过使用低成本原料经简单一锅反应制备.作为氧化组分的高氯酸根阴离子和作为燃料组分的还原性有机阳离子交替紧密堆积于钙钛矿结构中,使该类化合物不仅有比目前军用含能炸药(例如RDX和HMX)更优异的爆炸性能,而且有更高的稳定性;其中无金属组分的分子钙钛矿含能化合物具有与CL-20相当的爆炸性能以及更高的比冲(约344秒).这种将低成本有机燃料组分和氧化剂组分组装在高对称性三元晶体结构的分子组装策略为设计有实用前景的含能材料提供了新思路.
引文
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2 Zhang C,Sun C,Hu B,et al.Synthesis and characterization of the pentazolate anion cyclo-N5ˉin(N5)6(H3O)3(NH4)4Cl.Science,2017,355:374-376
3 Xu Y,Wang Q,Shen C,et al.A series of energetic metal pentazolate hydrates.Nature,2017,549:78-81
4 Bélanger-Chabot G,Rahm M,Haiges R,et al.Ammonia-(dinitramido)boranes:High-energy-density materials.Angew Chem Int Ed,2015,54:11730-11734
5 Fischer D,Gottfried JL,Klap?tke TM,et al.Synthesis and investigation of advanced energetic materials based on bispyrazolylmethanes.Angew Chem Int Ed,2016,55:16132-16135
6 Zhang W,Zhang J,Deng M,et al.A promising high-energydensity material.Nat Commun,2017,8:181
7 Agrawal JP.High Energy Materials:Propellants,Explosives and Pyrotechnics.Weinheim:Wiley-VCH Verlag Gm BH&Co.KGa A,2010
8 Tang Y,Kumar D,Shreeve J’M.Balancing excellent performance and high thermal stability in a dinitropyrazole fused 1,2,3,4-tetrazine.J Am Chem Soc,2017,139:13684-13687
9 Hermann TS,Karaghiosoff K,Klap?tke TM,et al.Synthesis and characterization of 2,2’-dinitramino-5,5’-bi(1-oxa-3,4-diazole)and derivatives as economic and highly dense energetic materials.Chem Eur J,2017,23:12087-12091
10 Bolton O,Matzger AJ.Improved stability and smart-material functionality realized in an energetic cocrystal.Angew Chem Int Ed,2011,50:8960-8963
11 Landenberger KB,Bolton O,Matzger AJ.Energetic-energetic cocrystals of diacetone diperoxide(DADP):Dramatic and divergent sensitivity modifications via cocrystallization.J Am Chem Soc,2015,137:5074-5079
12 Zhang J,Shreeve JM.Time for pairing:cocrystals as advanced energetic materials.Cryst Eng Comm,2016,18:6124-6133
13 Bennion JC,Siddiqi ZR,Matzger AJ.A melt castable energetic cocrystal.Chem Commun,2017,53:6065-6068
14 Fischer N,Fischer D,Klap?tke TM,et al.Pushing the limits of energetic materials-the synthesis and characterization of dihydroxylammonium 5,5’-bistetrazole-1,1’-diolate.J Mater Chem,2012,22:20418-20422
15 Freis M,Klap?tke TM,Stierstorfer J,et al.Di(1H-tetrazol-5-yl)methane as neutral ligand in energetic transition metal complexes.Inorg Chem,2017,56:7936-7947
16 Tang Y,Gao H,Mitchell LA,et al.Syntheses and promising properties of dense energetic 5,5’-dinitramino-3,3’-azo-1,2,4-oxadiazole and its salts.Angew Chem Int Ed,2016,55:3200-3203
17 Yin P,Zhang J,Mitchell LA,et al.3,6-Dinitropyrazolo[4,3-c]pyrazole-based multipurpose energetic materials through versatile N-functionalization strategies.Angew Chem Int Ed,2016,55:12895-12897
18 Tang Y,Mitchell LA,Imler GH,et al.Ammonia oxide as a building block for high-performance and insensitive energetic materials.Angew Chem Int Ed,2017,56:5894-5898
19 Zhang L,Song KX,Zhang Z,et al.Insensitive ionic bio-energetic materials derived from amino acids.Sci Rep,2017,7:12744
20 Liu W,Liu WL,Pang SP.Structures and properties of energetic cations in energetic salts.RSC Adv,2017,7:3617-3627
21 Bushuyev OS,Brown P,Maiti A,et al.Ionic polymers as a new structural motif for high-energy-density materials.J Am Chem Soc,2012,134:1422-1425
22 Li S,Wang Y,Qi C,et al.3D energetic metal-organic frameworks:synthesis and properties of high energy materials.Angew Chem Int Ed,2013,52:14031-14035
23 Zhang J,Du Y,Dong K,et al.Taming dinitramide anions within an energetic metal-organic framework:A new strategy for synthesis and tunable properties of high energy materials.Chem Mater,2016,28:1472-1480
24 Zhang S,Yang Q,Liu X,et al.High-energy metal-organic frameworks(HE-MOFs):Synthesis,structure and energetic performance.Coord Chem Rev,2016,307:292-312
25 Chen D,Jing D,Zhang Q,et al.Study of six green insensitive high energetic coordination polymers based on alkali/alkali-earth metals and 4,5-bis(tetrazol-5-yl)-2H-1,2,3-triazole.Chem Asian J,2017,12:3141-3149
26 Wang Q,Wang S,Feng X,et al.A heat-resistant and energetic metal-organic framework assembled by chelating ligand.ACSAppl Mater Interfaces,2017,9:37542-37547
27 Wang S,Wang Q,Feng X,et al.Explosives in the cage:Metalorganic frameworks for high-energy materials sensing and desensitization.Adv Mater,2017,29:1701898
28 Bostr?m HLB,Hill JA,Goodwin AL.Columnar shifts as symmetry-breaking degrees of freedom in molecular perovskites.Phys Chem Chem Phys,2016,18:31881-31894
29 Sun L.Crystal crosslinking.Nat Chem,2015,7:684-685
30 Liu T,Zhou Y,Hu Q,et al.Fabrication of compact and stable perovskite films with optimized precursor composition in the fastgrowing procedure.Sci China Mater,2017,60:608-616
31 Ding J,Yan Q.Progress in organic-inorganic hybrid halide perovskite single crystal:growth techniques and applications.Sci China Mater,2017,60:1063-1078
32 Xue M,Zhou H,Xu Y,et al.High-performance ultraviolet-visible tunable perovskite photodetector based on solar cell structure.Sci China Mater,2017,60:407-414
33 Cheetham AK,Rao CNR.There’s room in the middle.Science,2007,318:58-59
34 Xu WJ,Du ZY,Zhang WX,et al.Structural phase transitions in perovskite compounds based on diatomic or multiatomic bridges.Cryst Eng Comm,2016,18:7915-7928
35 You YM,Liao WQ,Zhao D,et al.An organic-inorganic perovskite ferroelectric with large piezoelectric response.Science,2017,357:306-309
36 Chen SL,Zhang WX,Chen XM.The 9thNational Conference in Inorganic Chemistry-B Coordination Chemistry.Nanchang,2015
37 Hand Book of Chemistry and Physics.84thedition,Florida:CRCPress,Taylor&Francis Group,2004
38 M.Su?eska,EXPLO5 6.04;Zagreb,Croatia,2017
39 Feng G,Jiang X,Wei W,et al.High pressure behaviour and elastic properties of a dense inorganic-organic framework.Dalton Trans,2016,45:4303-4308
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