Highly Selective Sensing of CO, C6H6, and C7H8 Gases by Catalytic Functionalization with Metal Nanoparticles
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- 作者：Jae-Hun Kim ; Ping Wu ; Hyoun Woo Kim ; Sang Sub Kim
- 刊名：ACS Applied Materials & Interfaces
- 出版年：2016
- 出版时间：March 23, 2016
- 年：2016
- 卷：8
- 期：11
- 页码：7173-7183
- 全文大小：739K
- ISSN：1944-8252
文摘
We have fabricated multiple networked SnO2 nanowires and subsequently decorated them with uniformly distributed metal nanoparticles (NPs). The sensing tests indicated that the Pt-, Pd-, and Au-decorated SnO2 nanowires exhibited excellent sensing behavior, specifically for C7H8, C6H6, and CO gases, respectively. We discussed the associated sensing mechanisms in regard to the selective catalytic effects of metal NPs. In addition, by means of d-band theory, we explained the catalytic capabilities of each metal and proposed design principles for exploring new catalytic metals. The present study will pave the way for further development of high-selectivity sensors.